Journal
PROCESSES
Volume 10, Issue 5, Pages -Publisher
MDPI
DOI: 10.3390/pr10051032
Keywords
combustion; flames; nitric oxide; hydrogen; nitrous oxide; dilution
Categories
Funding
- Romanian Academy
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A computational study was conducted to investigate the effect of adding nitrogen to hydrogen-nitrous oxide flames at different initial pressures and temperatures. The results showed that increasing the initial pressure and temperature led to higher mass fractions of NO and flame temperature.
A computational study was conducted on the addition of nitrogen (0-60 vol%) to stoichiometric hydrogen-nitrous oxide flames at various initial pressures (1-10 bar) and temperatures (300-500 K), with a special emphasis on NO, which is a major pollutant that is generated by these flames. The detailed kinetic modeling of H-2-N2O-N-2 flames, which was performed using the GRI 3.0 mechanism, produced the structure of the H-2-N2O-N-2 flames for the temperature and mass fraction profiles of 53 species, which participated in 325 elementary reactions. The NO profiles that were computed by the detailed kinetic modeling followed the trend of experimental NO profiles that have been reported in the literature for laminar premixed flames at sub-atmospheric pressures. For the examined H-2-N2O-N-2 flames, an increase in initial pressure resulted in a significant reduction in the NO mass fraction of the burned gas. The increase in initial temperature was also accompanied by an increase in the mass fractions of the generated NO, as well as the flame temperature.
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