4.6 Article

Highly Active Ice-Nucleating Particles at the Summer North Pole

Journal

Publisher

AMER GEOPHYSICAL UNION
DOI: 10.1029/2021JD036059

Keywords

Arctic; ice-nucleating particles; ice; mixed-phase clouds

Funding

  1. European Research Council [648661 MarineIce]
  2. Natural Environment Research Council [NE/R009686/1, NE/T00648X/1]
  3. Swiss National Science Foundation [200021_169090]
  4. Swiss National Science Foundation Early Postdoc.Mobility
  5. Swiss Polar Institute
  6. Knut-and-Alice-Wallenberg Foundation [2016.0024]
  7. Bolin Centre for Climate Research
  8. Swedish Research Council [2016-03518, 824-2013-222, 2018-05045, 2015-05318, 2016-05100]
  9. Ymer-80 foundation
  10. The Ingvar Kamprad Chair - Ferring Pharmaceuticals
  11. Vinnova [2016-03518] Funding Source: Vinnova
  12. NERC [NE/R009686/1, NE/T00648X/1] Funding Source: UKRI
  13. Swiss National Science Foundation (SNF) [200021_169090] Funding Source: Swiss National Science Foundation (SNF)
  14. Swedish Research Council [2018-05045, 2015-05318, 2016-03518] Funding Source: Swedish Research Council

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The study found that during the summer of 2018, high concentrations of biological INPs were sporadically present at the North Pole. These concentrations sometimes reached levels similar to those recorded in mid-latitude locations strongly impacted by highly active biological INPs, in contrast to the Southern Ocean. Furthermore, using a balloon borne sampler, the study demonstrated that INP concentrations differed between the surface and higher in the boundary layer where clouds form. These findings suggest that Arctic climate is sensitive to transport from regions that are already experiencing climate change.
The amount of ice versus supercooled water in clouds is important for their radiative properties and role in climate feedbacks. Hence, knowledge of the concentration of ice-nucleating particles (INPs) is needed. Generally, the concentrations of INPs are found to be very low in remote marine locations allowing cloud water to persist in a supercooled state. We had expected the concentrations of INPs at the North Pole to be very low given the distance from open ocean and terrestrial sources coupled with effective wet scavenging processes. Here we show that during summer 2018 (August and September) high concentrations of biological INPs (active at >-20 degrees C) were sporadically present at the North Pole. In fact, INP concentrations were sometimes as high as those recorded at mid-latitude locations strongly impacted by highly active biological INPs, in strong contrast to the Southern Ocean. Furthermore, using a balloon borne sampler we demonstrated that INP concentrations were often different at the surface versus higher in the boundary layer where clouds form. Back trajectory analysis suggests strong sources of INPs near the Russian coast, possibly associated with wind-driven sea spray production, whereas the pack ice, open leads, and the marginal ice zone were not sources of highly active INPs. These findings suggest that primary ice production, and therefore Arctic climate, is sensitive to transport from locations such as the Russian coast that are already experiencing marked climate change.

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