4.8 Review

Wide-Bandgap Organic-Inorganic Lead Halide Perovskite Solar Cells

Journal

ADVANCED SCIENCE
Volume 9, Issue 14, Pages -

Publisher

WILEY
DOI: 10.1002/advs.202105085

Keywords

indoor photovoltaics; semitransparent perovskite solar cells; tandem solar cells; voltage loss; wide-bandgap perovskite

Funding

  1. Strategic Priority Research Program of the Chinese Academy of Sciences [XDA17040506]
  2. National Nature Science Foundation of China [21805274, U20A20252, 21908013]
  3. Innovation Fund Project of Dalian Institute of Chemical Physics [DICP I202025, DICP I202032]
  4. Cooperation Foundation of Dalian National Laboratory for Clean Energy of the Chinese Academy of Sciences [DNL202015]
  5. Natural Science Foundation of Liaoning Province [2021-MS-016, 20180550656]
  6. National Key Research Program of China [2016YFA0202403]
  7. Youth Science and Technology Star Project of Dalian [2021RQ121]
  8. 111 Project [B1404]
  9. Doctor Startup Foundation of Dalian Polytechnic University [6102072032]
  10. Project of Knowledge Innovation Engineering [Y261261606]

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This review summarizes the progress of wide-bandgap mixed halide perovskite solar cells and discusses their diverse applications in different fields and the challenges they face.
Under the groundswell of calls for the industrialization of perovskite solar cells (PSCs), wide-bandgap (>1.7 eV) mixed halide perovskites are equally or more appealing in comparison with typical bandgap perovskites when the former's various potential applications are taken into account. In this review, the progress of wide-bandgap organic-inorganic hybrid PSCs-concentrating on the compositional space, optimization strategies, and device performance-are summarized and the issues of phase segregation and voltage loss are assessed. Then, the diverse applications of wide-bandgap PSCs in semitransparent devices, indoor photovoltaics, and various multijunction tandem devices are discussed and their challenges and perspectives are evaluated. Finally, the authors conclude with an outlook for the future development of wide-bandgap PSCs.

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