Journal
ADVANCED ELECTRONIC MATERIALS
Volume 8, Issue 6, Pages -Publisher
WILEY
DOI: 10.1002/aelm.202200036
Keywords
CoFe; O-2; (4); magnetoelectric coupling; vertically aligned nanocomposite; YFeO; (3)
Funding
- MRSEC Program of the National Science Foundation [DMR-1419807]
- National Science Foundation [ECS-0335765]
- Army Research Office [W911-NF-19-2-0119]
- MIT MathWorks Engineering Fellowships
- National Natural Science Foundation of China [52102135]
- State Key Laboratory of New Ceramic and Fine Processing, Tsinghua University [KF202103]
- Fundamental Research Funds for the Central Universities (Nankai University) [023-63213099]
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Researchers have successfully observed the self-assembled vertically aligned nanocomposites consisting of ferromagnetic pillars embedded in a ferroelectric matrix, and found that strain-mediated magnetoelectric coupling effect exists in this structure, which provides a new geometric configuration for studying magnetoelectric coupling based on strain-coupled magnetostrictive and piezoelectric effects.
Self-assembled two-phase vertically aligned nanocomposites consisting of ferromagnetic pillars embedded in a ferroelectric matrix provide an attractive geometry for observing magnetoelectric coupling based on the strain-coupled magnetostrictive and piezoelectric effects at the interfaces. In perovskite-spinel nanocomposites the ferroelectric phase typically consists of BiFeO3, BaTiO3 or Pb(Zr,Ti)O-3. Here, the ferroelectric phase is Y-rich YFeO3 which exhibits ferroelectricity originating from the local inversion symmetry breaking caused by Y-Fe antisite defects. Coherent interfaces observed between Y-rich YFeO3 and a magnetic spinel CoFe2O4 in a vertically aligned nanocomposite enable strain-mediated magnetoelectric coupling at room temperature, confirming the ferroelectricity and piezoelectricity in Y-rich YFeO3 and extending the range of magnetoelectric nanocomposite compositions.
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