4.7 Article

Thermal Conductivity of GaAs Nanowire Arrays Measured by the 3ω Method

Journal

NANOMATERIALS
Volume 12, Issue 8, Pages -

Publisher

MDPI
DOI: 10.3390/nano12081288

Keywords

nanowire; twinning superlattice; thermal conductivity; thermoelectric

Funding

  1. Natural Sciences and Engineering Research Council of Canada [RGPIN-2018-04015]

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This study utilized the three omega method to measure the thermal conductivity of two GaAs nanowire arrays with different crystal structures. The results showed that the nanowires with a twinning superlattice structure had a thermal conductivity nearly an order of magnitude lower than that of the bulk material.
Vertical nanowire (NW) arrays are the basis for a variety of nanoscale devices. Understanding heat transport in these devices is an important concern, especially for prospective thermoelectric applications. To facilitate thermal conductivity measurements on as-grown NW arrays, a common NW-composite device architecture was adapted for use with the 3 omega method. We describe the application of this technique to obtain thermal conductivity measurements on two GaAs NW arrays featuring similar to 130 nm diameter NWs with a twinning superlattice (TSL) and a polytypic (zincblende/wurtzite) crystal structure, respectively. Our results indicate NW thermal conductivities of 5.2 +/- 1.0 W/m-K and 8.4 +/- 1.6 W/m-K in the two samples, respectively, showing a significant reduction in the former, which is the first such measurements on TSL NWs. Nearly an order of magnitude difference from the bulk thermal conductivity (similar to 50 W/m-K) is observed for the TSL NW sample, one of the lowest values measured to date for GaAs NWs.

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