4.6 Article

Novel Methodology to Visualize Biomass Processing Sustainability & Cellulose Nanofiber Product Quality

Journal

ACS SUSTAINABLE CHEMISTRY & ENGINEERING
Volume 10, Issue 11, Pages 3623-3632

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acssuschemeng.1c08476

Keywords

cellulose nanofibre; quality; sustainability; sorghum; nanopaper; data visualization

Funding

  1. University of Queensland
  2. Grains Research and Development Corporation (GRDC)
  3. Australian Government

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One of the key challenges in the industrial translation of cellulose nanofiber (CNF) materials is the appropriate characterization and evaluation of product quality. The study explores the development of statistical methodologies to investigate quality and sustainability, including a visualization tool for processing sustainability evaluation, correlation analysis of biomass composition with processing sustainability and nanopaper performance, and a user-defined quality ranking methodology. The versatile framework enhances data analysis and assists researchers in elucidating material performance relationships and advancing the industrial translation of CNF products.
One of the key challenges for the industrial translation of cellulose nanofiber (CNF) materials is appropriate characterization and evaluation of product quality. Characterization of CNF properties is difficult because direct nanofiber assessment is largely unreliable and unscalable, while indirect characterization is often inaccurate and unable to be generalized across different biomass sources, processing routes, and final product or component formats. In addition, quality is an ambiguous term that is difficult to define, encompassing material performance, processing sustainability, and any aspects impacting economic viability of industrial production, dependent on the application in question. Using existing data on CNF produced from sorghum biomass, we explored the development of versatile statistical methodologies as a framework to investigate quality and sustainability, including: (a) a novel visualization tool for the evaluation of biomass processing sustainability (Processing Sustainability Triangle); (b) correlation analysis of biomass chemical composition with metrics relating to processing sustainability and nanopaper performance; and (c) an application-tunable Quality Ranking methodology based on a user-defined definition, as built through structural equation modeling. Versatility of the framework allows researchers and technologists to map the statistical methodology onto their experimental system of interest, enhancing data analysis through visualization. Ultimately,more sophisticated techniques for evaluation of product quality and processing sustainability will assist researchers to elucidate relationships in biomass-derived materialperformance and advance the industrial translation of CNF products.

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