4.8 Review

Buried Interface Modification in Perovskite Solar Cells: A Materials Perspective

Journal

ADVANCED ENERGY MATERIALS
Volume 12, Issue 20, Pages -

Publisher

WILEY-V C H VERLAG GMBH
DOI: 10.1002/aenm.202104030

Keywords

defect passivation; interface; perovskite solar cells; stability

Funding

  1. University Grant Council of the University of Hong Kong [202011159254]
  2. General Research Fund from the Research Grants Council (RGC) of Hong Kong Special Administrative Region, China [17200518, 17201819, 17211220, 17200021]
  3. Collaborative Research Grant from the Research Grants Council (RGC) of Hong Kong Special Administrative Region, China [C5037-18G, C7035-20G]

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This article examines the latest progress in modifying the buried interface of organic-inorganic hybrid perovskite solar cells (PSCs) to enhance their performance and stability. It discusses the use of various materials and techniques and provides valuable insights for achieving higher power conversion efficiency in PSCs and interface adjustment in other layered structure heterojunction devices.
Organic-inorganic hybrid perovskite solar cells (PSCs) are promising third-generation solar cells. They exhibit high power conversion efficiency (PCE) and, in theory, can be manufactured with less energy than several more established photovoltaic technologies, particularly solution-processed PSCs. Various materials have been widely utilized to modify the buried bottom interface to improve the performance and long-term stability of PSCs. Here, the latest progress in modifying the buried interface to enhance the performance and stability of PSCs is examined from a materials standpoint, which is classified into inorganic salts, the organic molecular and polymer, carbon materials, perovskite-related materials, and 2D materials. This material perspective is useful in determining the tactics for achieving the theoretical PCE value of PSCs. It also serves as a solid reference of interface adjustment for other layered structure heterojunction devices.

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