4.8 Article

High-Frequency Light Rectification by Nanoscale Plasmonic Conical Antenna in Point-Contact-Insulator-Metal Architecture

Journal

ADVANCED ENERGY MATERIALS
Volume 12, Issue 15, Pages -

Publisher

WILEY-V C H VERLAG GMBH
DOI: 10.1002/aenm.202103785

Keywords

energy harvesting; metal-insulator-metal diodes; optical rectificators; plasmonic diodes

Funding

  1. NSFC project [32071317]
  2. European Space Agency, ARIADNA grant
  3. National Science Foundation [IIP-1941227]
  4. H2020 FET-Open Program [964995]
  5. Istituto Italiano di Tecnologia within the CRUI-CARE Agreement

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Efforts have been made to develop efficient high-frequency rectifying antennas for light harvesting and photodetection applications, but there have been challenges in understanding the underlying physics and limitations in fabrication techniques. This study demonstrates a new type of rectifying antenna based on plasmonic carrier generation, which shows improved current generation and high efficiency at 280 THz (1064 nm).
Numerous efforts have been undertaken to develop rectifying antennas operating at high frequencies, especially dedicated to light harvesting and photodetection applications. However, the development of efficient high frequency rectifying antennas has been a major technological challenge both due to a lack of comprehension of the underlying physics and limitations in the fabrication techniques. Various rectification strategies have been implemented, including metal-insulator-metal traveling-wave diodes, plasmonic nanogap optical antennas, and whisker diodes, although all show limited high-frequency operation and modest conversion efficiencies. Here a new type of rectifying antenna based on plasmonic carrier generation is demonstrated. The proposed structure consists of a resonant metallic conical nano-antenna tip in contact with the oxide surface of an oxide/metal bilayer. The conical shape allows for an improved current generation based on plasmon-mediated electromagnetic-to-electron conversion, an effect exploiting the nanoscale-tip contact of the rectifying antenna, and proportional to the antenna resonance and to the surface-electron scattering. Importantly, this solution provides rectification operation at 280 THz (1064 nm) with a 100-fold increase in efficiency compared to previously reported results. Finally, the conical rectifying antenna is also demonstrated to operate at 384 THz (780 nm), hence paving a way toward efficient rectennas toward the visible range.

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