Journal
SYNTHESIS-STUTTGART
Volume 54, Issue 21, Pages 4673-4682Publisher
GEORG THIEME VERLAG KG
DOI: 10.1055/a-1829-0262
Keywords
chemodivergent reactions; [3+3] and [3+2] cycloadditions; azomethine ylide; cyclopropenone
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Funding
- Ministerio de Ciencia e Innovacion (MICINN)
- Fondo Europeo de Desarrollo Regional (FEDER, UE) [PGC2018-098660-B-100]
- Ministerio de Educacion Cultura y Deportes
- MICINN
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Chemodivergent cycloadditions of azomethine ylides with diphenylcyclopropenone have been developed, involving either Cu-catalyzed [3+3] or Ag-catalyzed [3+2] processes. These reactions provide a highly efficient method for the preparation of aromatic substituted dihydropyridinones and dihydropyrrolones with excellent regio and diastereoselectivities.
Chemodivergent cycloadditions of azomethine ylides with diphenylcyclopropenone involving either Cu-catalyzed [3+3] or Ag-catalyzed [3+2] processes have been developed. These transformations provide a highly efficient method for the preparation of a variety of aromatic substituted dihydropyridinones and dihydropyrrolones with excellent regio and diasteroselectivities.
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