Journal
ORGANIC LETTERS
Volume 24, Issue 21, Pages 3797-3801Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.2c01330
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Funding
- National Science Foundation of China [NSF 22171108]
- Guangxi Key Laboratory of Agricultural Resources Chemistry and Biotechnology [2020KF01]
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This article describes the development of a general strategy for the silylation of N-heteroaromatics and unsaturated benzamides by rationally designing an efficient organic photocatalyst. The process is characterized by its simplicity, mild reaction conditions, and utilization of readily prepared naphthalimide (NI)-based organic photocatalysts. Importantly, both inert trialkylhydrosilanes and arylhydrosilanes are compatible with this protocol.
Described herein is the development of a general strategy for the silylation of N-heteroaromatics and unsaturated benzamides via the rational designing of an efficient organic photocatalyst. The process features operational simplicity, mild reaction conditions, and the use of readily prepared naphthalimide (NI)-based organic photocatalysts. Notably, both inert trialkylhydrosilanes and arylhydrosilanes are well tolerated with this protocol.
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