4.8 Article

Correlated Hofstadter spectrum and flavour phase diagram in magic-angle twisted bilayer graphene

Journal

NATURE PHYSICS
Volume 18, Issue 7, Pages 825-+

Publisher

NATURE PORTFOLIO
DOI: 10.1038/s41567-022-01589-w

Keywords

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Funding

  1. US Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES) [DE-SC0021238]
  2. Stanford University Terman Fellowship
  3. Alfred P. Sloan Foundation Fellowship
  4. MEXT, Japan [JPMXP0112101001]
  5. JSPS KAKENHI [JP20H00354]
  6. Department of Energy, Office of Basic Energy Sciences [DEAC02-76SF00515]
  7. Stanford Graduate Fellowship
  8. Marvin Chodorow Postdoctoral Fellowship of the Applied Physics Department, Stanford University
  9. Gordon and Betty Moore Foundation's EPiQS Initiative [GBMF 4302, GBMF 8686]
  10. NSF [DMR-2111379]
  11. National Science Foundation [ECCS-2026822]
  12. U.S. Department of Energy (DOE) [DE-SC0021238] Funding Source: U.S. Department of Energy (DOE)

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This study examines the phase diagram of isospin polarization in magic-angle twisted bilayer graphene and discovers multiple many-body quantum phases and topological states in narrow energy bands, providing insights into the transitions between these states and their interplay with interactions and symmetry breaking.
In magic-angle twisted bilayer graphene, the moire superlattice potential gives rise to narrow electronic bands that support a multitude of many-body quantum phases. Further richness arises in the presence of a perpendicular magnetic field, where the interplay between moire and magnetic length scales leads to fractal Hofstadter subbands. In this strongly correlated Hofstadter platform, multiple experiments have identified gapped topological and correlated states, but little is known about the phase transitions between them in the intervening compressible regimes. Here we simultaneously unveil sequences of broken-symmetry Chern insulators and resolve sharp phase transitions between competing states with different topological quantum numbers and different occupations of the spin-valley flavour. Our measurements determine the energy spectrum of interacting Hofstadter subbands in magic-angle twisted bilayer graphene and map out the phase diagram of flavour occupancy. In addition, we observe full lifting of the degeneracy of the zeroth Landau levels together with level crossings, indicating moire valley splitting. We propose a unified flavour polarization mechanism to understand the intricate interplay of topology, interactions and symmetry breaking as a function of density and applied magnetic field in this system. In graphene, the spin and valley degrees of freedom combine into a higher-order isospin. Now, a full map of the phase diagram of this isospin is measured in the moire bands of twisted bilayer graphene.

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