4.8 Article

Perovskite: Scintillators, direct detectors, and X-ray imagers

Journal

MATERIALS TODAY
Volume 55, Issue -, Pages 110-136

Publisher

ELSEVIER SCI LTD
DOI: 10.1016/j.mattod.2022.04.009

Keywords

Perovskite; Scintillator; Direct detector; High-energy radiation; X-ray imaging; film phototransistor (TFT) arrays; amorphous Si photodiodes

Funding

  1. National Research Founda-tion (NRF) of Korea [2021R1A2B5B01001796, 2021R1F1A1062672, 2021R1F1A1062528, 2021R1A4A5031805]
  2. Technology Innovation Program [20013597]
  3. Ministry of Trade, Industry Energy
  4. National Research Foundation of Korea [2021R1F1A1062672, 2021R1F1A1062528] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)

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Halide perovskites are promising materials in various applications such as solar energy, optoelectronics, and medical imaging. With their excellent performance and low cost, halide perovskites could potentially replace traditional materials and play a significant role in high-energy radiation detection.
Halide perovskites (HPs) are used in various applications, including solar cells, light-emitting diodes, lasers, and photodetectors. These materials have recently received a great deal of attention as highenergy radiation detectors and scintillators due to their excellent light yield, mobility-lifetime product (ms), and X-ray sensitivity. In addition, due to their solution-processability and low cost, perovskite materials could be used to produce thick perovskite films across wide areas, allowing for low-dose X-ray imaging. Perovskite-based scintillators and detectors could eventually replace commercialized products like thallium-doped cesium iodide (CsI:Tl) and amorphous silicon (Si). Here, we review all of the key properties of HPs, the relevant terminology necessary for radiation detection and scintillation, the physical mechanisms underlying their operation, the fabrication process, and perovskite crystals and thin-films of varying dimensionality used for high-energy radiation detection. We also cover the critical issues and solutions that HPs as detectors, scintillators, and imagers face.

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