4.7 Article

Performance enhancement of soft-PZT5 piezoelectric ceramics using poling technique

Journal

JOURNAL OF THE AMERICAN CERAMIC SOCIETY
Volume 105, Issue 7, Pages 4744-4750

Publisher

WILEY
DOI: 10.1111/jace.18433

Keywords

alternating current poling; direct current poling; piezoelectricity; PZT

Funding

  1. National Natural Science Foundation of China [11904362, 51902307, 11974349]
  2. Science and Technology Project of Fujian Province [2020H0038, 2021H0043]
  3. Key Research Program of the Chinese Academy of Sciences [ZDRW-CN-2021-3]

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This study reports the dielectric and piezoelectric properties of soft-PZT5 ceramics under direct current poling (DCP), alternating current poling (ACP), and ACP + DCP methods. The results show that the ACP + DCP treatment significantly improves the piezoelectric properties of soft-PZT5 ceramics at room temperature.
Pb(Zr1-xTix)O-3 (PZT) ceramics are the most widely used piezoelectric ceramics due to their excellent performance. It has been reported that the direct current poling (DCP) apply on alternating current poling (ACP) relaxor-PbTiO3 ferroelectric crystals can further improve the piezoelectric properties. Herein, we report the dielectric and piezoelectric properties of soft-PZT5 ceramics under DCP, ACP, and ACP + DCP methods. The piezoelectric coefficient d(33) of the soft-PZT5 ceramics was 560 pC/N using ACP+DCP at room temperature (RT), which is 4% higher than the ACP-treated sample (540 pC/N) and 24% higher than the DCP-treated sample (450 pC/N). The ideal poling temperatures of DCP and ACP were found to be 120 degrees C and 60 degrees C, showing optimal d(33) values of 540 pC/N and 565 pC/N, respectively. The ACP and ACP+DCP samples show the same aging trend. After 30 days of aging, the d(33) values of the DCP, ACP, and ACP+DCP soft-PZT5 ceramics were 415 pC/N, 500 pC/N, and 510 pC/N, respectively, showing decreases of 12%, 8%, and 9%, respectively. This work indicates that the ACP+DCP method is an effective method to improve the piezoelectric properties of soft-PZT5 ceramics.

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