Journal
JOURNAL OF ORGANIC CHEMISTRY
Volume 87, Issue 9, Pages 6179-6188Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.joc.2c00408
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Funding
- Sichuan Science and Technology Program [2021YFG0111]
- National Natural Science Foundation of China [22107082]
- Guangxi Science and Technology Development under the Central Government [2021ZYD0058, ZY20198020]
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In this study, novel complex C2-quaternary-indol-3-one units bearing versatile nitro groups were successfully developed from pseudo-indolones and alpha,beta-unsaturated nitroolefins through rhodium-catalyzed C-H activation/[3 + 2] spirocyclization. Notably, four diastereomers could be selectively obtained in the reaction by condition control.
Novel complex C2-quaternary-indol-3-one units bearing versatile nitro groups have been successfully developed frompseudo-indolones and alpha,beta-unsaturated nitroolefins through rhodium-catalyzed C-H activation/[3 + 2] spirocyclization. Notably,four diastereomers could be selectively obtained in the reaction by condition control
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