4.5 Article

Characteristics of spin-thermoelectric generators enhanced by incorporating liquid phase epitaxial Bi-substituted YIG films as a ferrimagnetic insulator

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DOI: 10.1016/j.jmmm.2022.169081

Keywords

LPE Bi-substituted YIG films; Growth-induced magnetic anisotropy; Magnetic damping; Spin-orbital coupling; Enhanced spin-thermoelectric voltage

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Liquid phase epitaxial Bi-substituted YIG films exhibit a large growth-induced magnetic anisotropy perpendicular to the film surface. The anisotropy depends on the melt composition and supercooling in the growth process. Even at a Bi content of 0, the film shows a significant anisotropy. The spin-orbital coupling enhances the thermal energy transfer and increases spin currents for spin-thermoelectric generation.
Liquid phase epitaxial (LPE) Bi-substituted YIG films exhibit a large growth-induced magnetic anisotropy (GIMA) perpendicular to the film surface. The GIMA depends on the melt composition and supercooling in the LPE growth. Our film shows a large K-u value of 0.1 x 10(4) J/m(3) even at a Bi content, x, of 0. We assume that GIMA enhances the spin-orbital coupling (SOC) in the local d-electron spins of Fe3+, and that the SOC-enhanced thermal energy transfer from the phonon system to the spin system increases spin currents in spin- thermoelectric (STE) generation. We discuss the characteristics of STE generators on the basis of data obtained from ferromagnetic resonance measurements.

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