4.7 Article

Ceramsite production using water treatment residue as main ingredient: The key affecting factors identification

Journal

JOURNAL OF ENVIRONMENTAL MANAGEMENT
Volume 308, Issue -, Pages -

Publisher

ACADEMIC PRESS LTD- ELSEVIER SCIENCE LTD
DOI: 10.1016/j.jenvman.2022.114611

Keywords

Drinking water treatment residuals; Recycle; Graduation; Remediation

Funding

  1. National Natural Science Foundation of China [51779244, 41907361]
  2. Natural Science Foundation of Jiangsu Province [BK20190107]
  3. Youth Innovation Promotion Association CAS

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Recycling drinking water treatment residue (DWTR) to make ceramsite can provide environmental and economic benefits in water environment remediation. The key parameter for ceramsite production is the sintering temperature. Ceramsites made from different DWTR have varying properties and require specific ingredients preparation. DWTR based ceramsite is identified as non-hazardous material and has the ability to adsorb heavy metals.
As an inevitable by-product of potable water production, drinking water treatment residue (DWTR) recycling to make ceramsite can provide both environmental and economic benefits in constructing filtration treatment system for water environment remediation. Given the varied properties of DWTR from different waterworks, this study aims to identify the key factors affecting ceramsite production from DWTR as main ingredient based on five different DWTR with using clay as the auxiliary material. The results showed that of sintering temperature (500-1000 ?), DWTR:clay ratio (5:5 to 9:1), sintering time (5-60 min), and granule diameter (5-15 mm), the sintering temperature was the key parameter. Increasing temperatures from 500 to 1000 ? gradually promoted DWTR sintering by enhancing Si and Al crystallization, which typically increased the formation of SiO2 and CaAl2Si2O8 crystals in ceramsite. Ceramsites made from different DWTR tended to have different properties, mainly resulting from varied contents of Si (20.2%-48.6%), K (0.0894%-2.39%), Fe (4.56%-14.3%), and loss on ignition (11.7%-39.5%). During ingredients preparation to produce up-to-standard ceramsite, supplying additional Si and diluting loss on ignition were necessary for all DWTR, while supplying K and diluting Fe may be required for specific DWTR, due to the potential varied DWTR compositions caused by different water production processes applied (e.g., type of flocculants). Further toxicity characteristic leaching procedure analysis indicated the increased leaching of Cu. However, DWTR based ceramsite was identified as non-hazardous material; even, sintering treatment reduced the leachability of Ba, Be, Cd, and Cr. DWTR based ceramsite also had relatively high specific surface area (22.1-50.5 m(2)/g) and could adsorb Cd, Cu, and Pb from solution. Overall, based on appropriate management, DWTR can be recycled as the main ingredient in the production of ceramsite for water environment remediation.

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