Journal
JOURNAL OF ELECTROANALYTICAL CHEMISTRY
Volume 915, Issue -, Pages -Publisher
ELSEVIER SCIENCE SA
DOI: 10.1016/j.jelechem.2022.116353
Keywords
CO2RR; Cu nanoparticles loaded on nitrogen-doped carbon; CH4; Pyridinic N
Categories
Funding
- National Key R&D Program of China [2020YFA0710200]
- National Natural Science Foundation of China [22072046]
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In this study, Cu nanoparticles loaded on nitrogen-doped carbon materials were prepared for the electrochemical reduction of CO2, showing good selectivity for C1 and significant catalytic activity.
Electrochemical reduction of CO2 to produce valuable carbon-based fuels can solve the energy problem and achieve carbon neutrality. Herein, a series of Cu nanoparticles loaded on nitrogen-doped carbon materials (Cu@NC) for the electrochemical reduction of CO2 are prepared and show good selectivity for C1. Abundant pyridinic N and high dispersion of Cu nanoparticles enhance the electrocatalytic activity. The highest C1 Faradaic efficiency (FE) of 53% is obtained on Cu@NC-3, including FE of 30% for CH4.
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