Ibuprofen degradation by a synergism of facet-controlled MIL-88B(Fe) and persulfate under simulated visible light

Article Engineering, Environmental

Photocatalytic Cr(VI) reduction over MIL-101(Fe)-NH2 immobilized on alumina substrate: From batch test to continuous operation

Qian Zhao et al.

Summary: The MA photocatalyst prepared via hydrothermal immobilization method can achieve efficient Cr(VI) reduction under white light, showing potential for continuous operation in fixed-bed reactors.

CHEMICAL ENGINEERING JOURNAL (2022)

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Article Engineering, Environmental

Defects controlled by acid-modulators and water molecules enabled UiO-67 for exceptional toluene uptakes: An experimental and theoretical study

Xiaodong Zhang et al.

Summary: This paper presents a facile defect-engineering approach using monocarboxylic acid modulators to enhance toluene uptake in UiO-67 MOFs. The presence of water molecules was found to creatively promote adsorption behavior of defective UiO-67, leading to structural changes and stronger interaction between toluene and the material. The study highlights the potential of defect-tunable MOFs as promising materials for gas adsorption applications.

CHEMICAL ENGINEERING JOURNAL (2022)

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Article Chemistry, Physical

Bicarbonate-enhanced iron-based Prussian blue analogs catalyze the Fenton-like degradation of p-nitrophenol

Yiqiong Yang et al.

Summary: Four iron-based Prussian blue analogs were prepared and Co-Fe PBA was found to exhibit excellent degradation performance for p-nitrophenol. This study presents a promising green heterogeneous catalyst for the degradation of emerging contaminants.

JOURNAL OF COLLOID AND INTERFACE SCIENCE (2022)

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Article Chemistry, Physical

Uniform platinum nanoparticles loaded on Universitetet i Oslo-66 (UiO-66): Active and stable catalysts for gas toluene combustion

Yiqiong Yang et al.

Summary: Highly dispersed Pt nanoparticles supported UiO-66 catalysts were successfully prepared and their thermal catalytic performances were evaluated by toluene degradation. The catalysts exhibited good catalytic performance in high weight hourly space velocity, stability, and water resistance test, and their performance was enhanced in the reusability test, possibly due to a Pt-0-PtO synergistic catalytic mechanism and phase transition between Pt-0 and PtO.

JOURNAL OF COLLOID AND INTERFACE SCIENCE (2022)

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Review Engineering, Environmental

Critical review of perovskite-based materials in advanced oxidation system for wastewater treatment: Design, applications and mechanisms

Naipeng Lin et al.

Summary: Perovskite, with its low cost, high stability, excellent catalytic activity, diverse structure, and strong conversion adaptability, has attracted widespread attention in the field of modern environmental catalysis. By coupling perovskite catalysts with advanced oxidation processes, it is possible to effectively remove organic pollutants from wastewater.

JOURNAL OF HAZARDOUS MATERIALS (2022)

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Article Engineering, Environmental

Insights into the mechanism of enhanced peroxymonosulfate degraded tetracycline using metal organic framework derived carbonyl modified carbon-coated Fe0

Yiqiong Yang et al.

Summary: Tetracycline (TC) degradation in water was successfully achieved using carbonyl-modified carbon-coated Fe0 as an activator for peroxymonosulfate (PMS). The Fe0 continuously activated PMS, while carbon facilitated electron transportation and the carbonyl group on the carbon surface acted as the active site. This study demonstrates the promising potential of this novel material for removing antibiotics from water.

JOURNAL OF HAZARDOUS MATERIALS (2022)

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Article Chemistry, Physical

Adsorption property of fluoride in water by metal organic framework: Optimization of the process by response surface methodology technique

Yiqiong Yang et al.

Summary: In this study, three types of metal-organic frameworks adsorbents were used to remove fluoride from wastewater, and the adsorption conditions were optimized. Among them, aluminum metal-organic frameworks showed the best adsorption performance. The study also revealed that pH was the most important factor influencing fluoride removal by one of the metal-organic frameworks.

SURFACES AND INTERFACES (2022)

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Review Chemistry, Physical

Preparation of modified zirconium-based metal-organic frameworks (Zr-MOFs) supported metals and recent application in environment: A review and perspectives

Quanxin Du et al.

Summary: This review summarizes the applications of zirconium-based metal-organic frameworks (Zr-MOFs) in adsorption, photocatalysis, and catalytic removal of pollutants. It also discusses the combination of metals with Zr-MOFs, their structure characteristics, and future prospects.

SURFACES AND INTERFACES (2022)

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Article Chemistry, Multidisciplinary

Site Sensitivity of Interfacial Charge Transfer and Photocatalytic Efficiency in Photocatalysis: Methanol Oxidation on Anatase TiO2 Nanocrystals

Cong Fu et al.

Summary: The study found that Ti sites exposed on {001} facets of anatase TiO2 nanocrystals have a significant impact on the photocatalytic oxidation of methanol, with CH3O(a)(Ti4c) showing high efficiency in photocatalytic oxidation rates.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Physical

The promoting effect of H2O on rod-like MnCeOx derived from MOFs for toluene oxidation: A combined experimental and theoretical investigation

Xiaodong Zhang et al.

Summary: The 3Mn2Ce catalyst shows superior catalytic performance and stability under high humidity conditions, mainly attributed to the formation of a solid solution between Ce and Mn species and better reducibility. The introduction of water can promote toluene mineralization by activating oxygen vacancies and facilitating the degradation pathway of toluene.

APPLIED CATALYSIS B-ENVIRONMENTAL (2021)

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Article Engineering, Environmental

Strategies to enhance catalytic performance of metal-organic frameworks in sulfate radical-based advanced oxidation processes for organic pollutants removal

Xuedong Du et al.

Summary: This review systematically summarizes the basic strategies to enhance the catalytic performance of metal-organic frameworks (MOFs) in sulfate radical (SO4 center dot-)-based advanced oxidation processes (SR-AOPs), including modulating metal clusters and organic ligands, as well as introducing optimization, modification, and composite strategies. The preparation methods, characterizations, catalytic performances, and mechanisms of several typical MOFs are highlighted in this review. The prospects and challenges of MOFs applied to SR-AOPs are also discussed.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Environmental Sciences

Bifunctional Bi12O17Cl2/MIL-100(Fe) composites toward photocatalytic Cr(VI) sequestration and activation of persulfate for bisphenol A degradation

Chen Zhao et al.

Summary: BM200 composite showed efficient Cr(VI) sequestration and PS activation under white light, outperforming the pristine materials. Addition of SOAs significantly improved photocatalytic reduction efficiency, and BPA degradation was achieved over a wide pH range.

SCIENCE OF THE TOTAL ENVIRONMENT (2021)

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Article Chemistry, Physical

Boron nitride nanosheets decorated MIL-53(Fe) for efficient synergistic ibuprofen photocatalytic degradation by persulfate activation

Ning Liu et al.

Summary: In this study, BNNs and MIL-53(Fe) composites were successfully prepared using a one-step hydrothermal method, and their catalytic performance in the photodegradation of IBP was investigated. Among the composites, BNFe-3 showed the highest activity in IBP degradation and maintained strong stability after four cycles. The enhanced decomposition rate of IBP was attributed to the activation of PS and improved electron transfer efficiency between BNNs and MIL-53(Fe).

JOURNAL OF COLLOID AND INTERFACE SCIENCE (2021)

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Article Environmental Sciences

Biodegradation of salicylic acid, acetaminophen and ibuprofen by bacteria collected from a full-scale drinking water biofilter

Mahmudul Hasan et al.

Summary: This study investigated the biodegradation of pharmaceuticals and a natural organic surrogate by bacteria seeded from backwash water in the presence of oxygen. The results showed efficient removal of salicylic acid, moderate removal of acetaminophen, and poor removal of ibuprofen. ATP levels in the reactor were found to be correlated with biodegradation rates, oxygen uptake rate, and extracellular polymeric substances.

JOURNAL OF ENVIRONMENTAL MANAGEMENT (2021)

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Article Environmental Sciences

Adsorption removal of ibuprofen and naproxen from aqueous solution with Cu-doped Mil-101(Fe)

Ping Xiong et al.

Summary: A new Cu-doped Mil-101(Fe) material was successfully synthesized and applied for the removal of ibuprofen and naproxen from water. The adsorption performance of Cu-doped Mil-101(Fe) was effective for both drugs and could be regenerated for repeated use.

SCIENCE OF THE TOTAL ENVIRONMENT (2021)

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Article Engineering, Chemical

Insights into water film DBD plasma driven by pulse power for ibuprofen elimination in water: performance, mechanism and degradation route

Zhen Li et al.

Summary: Efficient abatement technology for drugs and personal care products (PPCPs) is crucial in preventing their discharge into natural water environments. This study investigated the elimination of ibuprofen (IBP) using a water film dielectric barrier discharge (DBD) plasma system, driven by pulse power. Factors such as input power, frequency, duty ratio, and solution flowrate were found to influence the degradation of IBP.

SEPARATION AND PURIFICATION TECHNOLOGY (2021)

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Article Engineering, Environmental

Facet-controlled activation of persulfate by goethite for tetracycline degradation in aqueous solution

Min Yang et al.

Summary: This study utilized goethite with different exposed facets as catalysts for PS activation, finding that more {021} facet exposed goethite exhibited better catalytic performance due to its facilitation of generating active radicals to drive the degradation process. Advanced oxidation processes based on the activation of persulfate by facet-dependent goethite provide valuable insights for environmental catalysis.

CHEMICAL ENGINEERING JOURNAL (2021)

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Review Engineering, Environmental

Remediation of antibiotic wastewater by coupled photocatalytic and persulfate oxidation system: A critical review

Guanyi Chen et al.

Summary: This study provides a comprehensive overview of the PPOH system for antibiotic wastewater treatment, categorizing it into PPA, PAP, and CPPA systems. Through discussing the synergistic effects between photocatalysis and persulfate activation, the performance of the coupled oxidation systems and internal mechanisms for antibiotic degradation are summarized and analyzed, along with proposing conclusions and future prospects for the PPOH systems.

JOURNAL OF HAZARDOUS MATERIALS (2021)

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Article Chemistry, Physical

Photocatalysis-activated SR-AOP over PDINH/MIL-88A(Fe) composites for boosted chloroquine phosphate degradation: Performance, mechanism, pathway and DFT calculations

Xiao-Hong Yi et al.

Summary: PDINH/MIL-88A(Fe) composites were fabricated using a facile ball-milling strategy, showing outstanding degradation performance towards CQ under low power LED visible light. The activation of PDS over P25M175 and pristine MIL-88A contributed to boosted CQ degradation efficiency through direct and indirect electron transfer. Active radicals and singlet oxygen were found to participate in the CQ decomposition, with proposed degradation pathways and toxicity evaluations of intermediates.

APPLIED CATALYSIS B-ENVIRONMENTAL (2021)

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Article Chemistry, Physical

Degradation of benzophenone-4 by peroxymonosulfate activated with microwave synthesized well-distributed CuBi2O4 microspheres: Theoretical calculation of degradation mechanism

Yiping Wang et al.

Summary: This study found that well-distributed CuBi2O4 microspheres with active sites and hydroxyl groups on the surface can effectively activate PMS to degrade BP-4. The degradation mechanism of BP-4 was proposed through theoretical calculations and intermediates identification, showing that radical addition reaction is the main pathway for BP-4 oxidation.

APPLIED CATALYSIS B-ENVIRONMENTAL (2021)

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Article Engineering, Environmental

MIL-88B(Fe)-coated photocatalytic membrane reactor with highly stable flux and phenol removal efficiency

Chechia Hu et al.

Summary: In this study, two photocatalytic membrane reactors (PMRs) were successfully developed for phenol degradation, with the PHMR system showing significantly enhanced phenol removal efficiency and stable flux, while the PFMR system had lower flux but demonstrated good recyclability and stability. Both systems exhibited promising potential as effective, feasible, and sustainable wastewater treatment systems.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Engineering, Environmental

Insights into the degradation mechanism of perfluorooctanoic acid under visible-light irradiation through fabricating flower-shaped Bi5O7I/ZnO n-n heterojunction microspheres

Yiqiong Yang et al.

Summary: The Bi5O2I/ZnO n-n heterojunction microspheres showed excellent photocatalytic performance in degrading PFOA, with photoproduction holes attacking the carboxylic groups of PFOA and transforming it into shorter chain perfluorocarboxylic acids. This photocatalyst has the potential to be an effective treatment for PFOA contamination.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Environmental Sciences

Simultaneous hydrogen production and ibuprofen degradation by green synthesized Cu2O/TNTAs photoanode

Chia-Hung Chen et al.

Summary: This study successfully produced clean energy hydrogen and removed pollutants simultaneously in water using the photoelectrochemical method. By modifying cuprous oxide on titanate nanotube arrays, the electron mobility was improved, leading to an effective reduction of electron-hole pair recombination rate, achieving ibuprofen degradation and hydrogen generation simultaneously.

CHEMOSPHERE (2021)

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Article Engineering, Environmental

Synergetic Molecular Oxygen Activation and Catalytic Oxidation of Formaldehyde over Defective MIL-88B(Fe) Nanorods at Room Temperature

Shuping Zhang et al.

Summary: Defective MIL-88B(Fe) nanorods are used as a catalyst for catalytic oxidation of formaldehyde by activating molecular oxygen at ambient temperature. The Fe-CUSs on the nanorods facilitate efficient O-2 activation and generation of ROSs, leading to the successful oxidation of formaldehyde with high mineralization efficiency. This study provides new insights into utilizing novel MOF catalysts for efficient O-2 activation and reliable indoor air purification at ambient temperature.

ENVIRONMENTAL SCIENCE & TECHNOLOGY (2021)

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Review Environmental Sciences

Sorptive and microbial riddance of micro-pollutant ibuprofen from contaminated water: A state of the art review

Sumona Show et al.

Summary: The continuous discharge of ibuprofen in local water systems has become a growing concern due to its adverse environmental effects. In order to prevent further pollution, adsorption and bioremediation are considered more cost-effective and energy efficient methods for ibuprofen removal.

SCIENCE OF THE TOTAL ENVIRONMENT (2021)

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Article Chemistry, Physical

Functionalized g-C3N4 sheets assisted synthesis of growth-oriented MIL-88B-Fe with rod-like structure: Upgrading framework photo-catalytic performance and stability

Xiaoyuan Liao et al.

APPLIED SURFACE SCIENCE (2020)

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Article Engineering, Environmental

Remarkably enhanced sulfate radical-based photo-Fenton-like degradation of levofloxacin using the reduced mesoporous MnO@MnOx microspheres

Anqi Wang et al.

CHEMICAL ENGINEERING JOURNAL (2020)

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Article Chemistry, Multidisciplinary

Metal-Organic Framework Derived Porous α-Fe2O3/C Nano-shuttles for Enhanced Visible-light Photocatalysis

Yingping Pang et al.

CHEMISTRYSELECT (2020)

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Article Engineering, Environmental

In situ photoreduction of structural Fe(III) in a metal-organic framework for peroxydisulfate activation and efficient removal of antibiotics in real wastewater

Renli Yin et al.

JOURNAL OF HAZARDOUS MATERIALS (2020)

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Article Engineering, Environmental

Rapid degradation of tetracycline hydrochloride by heterogeneous photocatalysis coupling persulfate oxidation with MIL-53(Fe) under visible light irradiation

Ying Zhang et al.

JOURNAL OF HAZARDOUS MATERIALS (2020)

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Article Engineering, Environmental

Nanofiltration in pilot scale for wastewater reclamation: Long-term performance and membrane biofouling characteristics

Rui Xu et al.

CHEMICAL ENGINEERING JOURNAL (2020)

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Article Environmental Sciences

Facile preparation of iron oxide doped Fe-MOFs-MW as robust peroxydisulfate catalyst for emerging pollutants degradation

Yongjie Wan et al.

CHEMOSPHERE (2020)

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Article Materials Science, Multidisciplinary

Magnetic Fe3O4@MIL-53(Fe) nanocomposites derived from MIL-53(Fe) for the photocatalytic degradation of ibuprofen under visible light irradiation

Ning Liu et al.

MATERIALS RESEARCH BULLETIN (2020)

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Article Environmental Sciences

Seasonal occurrence, removal and risk assessment of 10 pharmaceuticals in 2 sewage treatment plants of Guangdong, China

Ying Tang et al.

ENVIRONMENTAL TECHNOLOGY (2019)

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Article Engineering, Environmental

Photochemical treatment of tyrosol, a model phenolic compound present in olive mill wastewater, by hydroxyl and sulfate radical-based advanced oxidation processes (AOPs)

Melike Yalili Kilic et al.

JOURNAL OF HAZARDOUS MATERIALS (2019)

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Article Engineering, Environmental

Efficient mineralization of aqueous antibiotics by simultaneous catalytic ozonation and photocatalysis using MgMnO3 as a bifunctional catalyst

Jiang Lu et al.

CHEMICAL ENGINEERING JOURNAL (2019)

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Article Chemistry, Multidisciplinary

High-Rate, Tunable Syngas Production with Artificial Photosynthetic Cells

Hongwen Zhang et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2019)

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Photocatalytic oxidation of sulfamethoxazole in the presence of TiO2: Effect of matrix in aqueous solution on decomposition mechanisms

Rongfang Yuan et al.

CHEMICAL ENGINEERING JOURNAL (2019)

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Article Engineering, Environmental

In-situ fabrication of needle-shaped MIL-53(Fe) with 1T-MoS2 and study on its enhanced photocatalytic mechanism of ibuprofen

Ning Liu et al.

CHEMICAL ENGINEERING JOURNAL (2019)

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Article Materials Science, Multidisciplinary

Effect of synthesis conditions on the photocatalytic degradation of Rhodamine B of MIL-53(Fe)

Ning Liu et al.

MATERIALS LETTERS (2019)

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Review Environmental Sciences

Pharmaceuticals in freshwater aquatic environments: A comparison of the African and European challenge

Samuel Fekadu et al.

SCIENCE OF THE TOTAL ENVIRONMENT (2019)

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Article Chemistry, Physical

Replacement of Chromium by Non-Toxic Metals in Lewis-Acid MOFs: Assessment of Stability as Glucose Conversion Catalysts

Ralentri Pertiwi et al.

CATALYSTS (2019)

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Enhanced Generation of Reactive Oxygen Species under Visible Light Irradiation by Adjusting the Exposed Facet of FeWO4 Nanosheets To Activate Oxalic Acid for Organic Pollutant Removal and Cr(VI) Reduction

Jun Li et al.

ENVIRONMENTAL SCIENCE & TECHNOLOGY (2019)

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Article Engineering, Environmental

Degradation of Ofloxacin by Perylene Diimide Supramolecular Nanofiber Sunlight-Driven Photocatalysis

Ping Chen et al.

ENVIRONMENTAL SCIENCE & TECHNOLOGY (2019)

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Article Chemistry, Physical

Ultrathin graphene oxide encapsulated in uniform MIL-88A(Fe) for enhanced visible light-driven photodegradation of RhB

Ning Liu et al.

APPLIED CATALYSIS B-ENVIRONMENTAL (2018)

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Article Engineering, Environmental

Integration of plasmonic effect into spindle-shaped MIL-88A(Fe): Steering charge flow for enhanced visible-light photocatalytic degradation of ibuprofen

Wenyuan Huang et al.

CHEMICAL ENGINEERING JOURNAL (2018)

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Article Engineering, Environmental

Solar light driven degradation of norfloxacin using as-synthesized Bi3+ and Fe2+ co-doped ZnO with the addition of HSO5- : Toxicities and degradation pathways investigation

Noor S. Shah et al.

CHEMICAL ENGINEERING JOURNAL (2018)

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One-step prepared cobalt-based nanosheet as an efficient heterogeneous catalyst for activating peroxymonosulfate to degrade caffeine in water

Kun-Yi Andrew Lin et al.

JOURNAL OF COLLOID AND INTERFACE SCIENCE (2018)

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Chemistry of persulfates in water and wastewater treatment: A review

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Synthesis of sea urchin-like carbon nanotubes/porous carbon superstructures derived from waste biomass for treatment of various contaminants

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APPLIED CATALYSIS B-ENVIRONMENTAL (2017)

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ACS APPLIED MATERIALS & INTERFACES (2017)

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Oxidative degradation of TMAH solution with UV persulfate activation

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CHEMICAL ENGINEERING JOURNAL (2014)

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Occurrence of acidic pharmaceuticals and personal care products in Tuna River Basin: From waste to drinking water

Eric Carmona et al.

SCIENCE OF THE TOTAL ENVIRONMENT (2014)

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Iron-Based Metal-Organic Frameworks MIL-88B and NH2-MIL-88B: High Quality Microwave Synthesis and Solvent-Induced Lattice Breathing

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CRYSTAL GROWTH & DESIGN (2013)

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Application of magnetite-activated persulfate oxidation for the degradation of PAHs in contaminated soils

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CHEMOSPHERE (2012)

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New photocatalysts based on MIL-53 metal-organic frameworks for the decolorization of methylene blue dye

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JOURNAL OF HAZARDOUS MATERIALS (2011)

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Article Environmental Sciences

Occurrence and risk assessment of acidic pharmaceuticals in the Yellow River, Hai River and Liao River of north China

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SCIENCE OF THE TOTAL ENVIRONMENT (2010)

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Ibuprofen degradation by a synergism of facet-controlled MIL-88B(Fe) and persulfate under simulated visible light

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