4.7 Article

Effects of temperature gradients on magnetic anisotropy of SmCo based films

Journal

JOURNAL OF ALLOYS AND COMPOUNDS
Volume 898, Issue -, Pages -

Publisher

ELSEVIER SCIENCE SA
DOI: 10.1016/j.jallcom.2021.162900

Keywords

SmCo based films; Temperature gradients; Magnetic anisotropy

Funding

  1. National Natural Science Foundation of China [51901079, 51801047]
  2. Fundamental Research Funds for the Central Universities
  3. Nature Science Foundation of Guangdong Province [2018A030310406, 2020A1515010736]
  4. Guangzhou Municipal Science and Technology Program [202007020008, 202102020596]
  5. Zhongshan Collaborative Innovation Fund [2018C1001]
  6. Zhongshan Science and Technology Program [191007102629094]
  7. Yunfu Municipal Science and Technology Program [2020A090103]
  8. Opening Project of National Engineering Research Center for Powder Metallurgy of Titanium Rare Metals

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This study systematically investigates the effects of RTP treatment on the magnetic anisotropy of SmCo-based films. The results show that RTP treatment can improve the magnetic properties and enhance the contrast of magnetic domains.
The magnetic anisotropy of SmCo-based permanent magnetic thin films are generally controlled by introducing buffer layer or heating substrate. However, the design for the multi-layer thin film system is complicated and the thickness of SmCo is limited due to a short range of interfacial stress/strain between the buffer layer and SmCo layer. In this work, the effects of temperature gradients, generated by RTP (rapid thermal process), on the magnetic anisotropy of the SmCo-based films were systematically investigated. The results show that the as-deposited films exhibit amorphous state. The out-of-plane coercivity of RTP-treated films is strongly correlated with the heating rate, and its optimum value (2810 Oe) is larger than that of the CTA (conventional thermal annealing) treated films (1670 Oe). For the RTP-treated films, the intensity of characteristic diffraction peaks for in-plane oriented SmCo5 (200) and Sm2Co17 (300) decreases, together with reducing the roughness. Besides, the grain size is finer and the contrast of magnetic domains becomes stronger for the RTP-treated films due to that the easy axis of SmCo5/Sm2Co17 phase gradually changes from in-plane to out-of-plane direction. It is suggested that the RTP treatment with a shorter annealing time has beneficial effects on obtaining finer microstructure and improving the out-of-plane magnetic anisotropy of the SmCo-based films. This work provides a novel way to control the magnetic anisotropy via annealing temperature gradients for permanent magnetic thin films, compared with conventional methods, to induce the magnetic anisotropy. (C) 2021 Elsevier B.V. All rights reserved.

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