Periodate activated by manganese oxide/biochar composites for antibiotic degradation in aqueous system: Combined effects of active manganese species and biochar

Article Chemistry, Physical

Structure defined 2D Mo2C/2Dg-C3N4 Van der Waals heterojunction: Oriented charge flow in-plane and separation within the interface to collectively promote photocatalytic degradation of pharmaceutical and personal care products

Yin Zhou et al.

Summary: The research team has developed a 2D/2D Mo2C/g-C3N4 Van der Waals heterojunction photocatalyst that can efficiently degrade PPCPs, providing a green strategy for typical PPCPs removal.

APPLIED CATALYSIS B-ENVIRONMENTAL (2022)

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Article Engineering, Environmental

Collaborative optimization for the performance of ZnO/biochar composites on persulfate activation through plant enrichment-pyrolysis method

Ruyi Xu et al.

Summary: A novel method was used to prepare ZnO/biochar composites, which showed advantages in persulfate activation for tetracycline degradation compared to conventional methods. ZnO NPs promoted the formation of persistent free radicals (PFRs) and enhanced catalytic ability, while the high porosity and large specific surface area of biochar composites facilitated electron transfer efficiency.

CHEMICAL ENGINEERING JOURNAL (2022)

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Article Engineering, Environmental

Tailoring biochar for persulfate-based environmental catalysis: Impact of biomass feedstocks

Ge Song et al.

Summary: This paper provides a systematic review of the properties of biochar and the relationship between catalytic performance in PS-AOPs and biomass feedstocks, introducing the differences in physicochemical properties and activation path of different sourced biochars. It summarizes how tailoring biochar affects its activation efficiency and mechanism in PS-AOPs, and proposes suitable application scenarios, appropriate methods to improve catalytic performance, and prospects and challenges for the development of biochar in PS-AOPs.

JOURNAL OF HAZARDOUS MATERIALS (2022)

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Article Chemistry, Physical

Dual optimization approach to Mo single atom dispersed g-C3N4 photocatalyst: Morphology and defect evolution

Chen Zhang et al.

Summary: The study investigated an advanced photocatalyst based on N-vacancy tubular porous g-C3N4 decorated with atomically dispersed Mo, showing remarkable photocatalytic performance for tetracycline degradation under visible light irradiation. The large specific surface area of the tubular morphology contributes to suppress the agglomeration of Mo atoms, while the N defect induces the formation of specific stable Mo-2 C/2 N configuration.

APPLIED CATALYSIS B-ENVIRONMENTAL (2022)

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Article Engineering, Environmental

Non-radical mechanism and toxicity analysis of β-cyclodextrin functionalized biochar catalyzing the degradation of bisphenol A and its analogs by peroxydisulfate

Xuan-Yuan Pei et al.

Summary: This study investigated the degradation mechanisms and potential ecotoxicity of four bisphenols compounds, and found that modified biochar can trigger the degradation of bisphenol pollutants through electron transfer in PDS catalysis, reducing the production of toxic intermediates.

JOURNAL OF HAZARDOUS MATERIALS (2022)

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Article Environmental Sciences

Biochar Modified by Nano-manganese Dioxide as Adsorbent and Oxidant for Oxytetracycline

Lirong Feng et al.

Summary: The study investigated the adsorption properties of bamboo willow biochar loaded with nMnO2 on oxytetracycline, finding that MBC removed OTC more effectively than BC, with the best performance at near-neutral pH conditions and minimal influence from factors like NaCl and NOM.

BULLETIN OF ENVIRONMENTAL CONTAMINATION AND TOXICOLOGY (2021)

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Review Chemistry, Multidisciplinary

Hydrothermal and Pyrolytic Conversion of Biomasses into Catalysts for Advanced Oxidation Treatments

Xi He et al.

Summary: This review introduces and compares two innovative biomass-based catalysts, HTCC and biochar, generated at different temperatures. HTCC is suitable for photocatalysis, while biochar is mainly used as an AOP catalyst for environmental treatment.

ADVANCED FUNCTIONAL MATERIALS (2021)

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Review Chemistry, Multidisciplinary

Environmental applications of carbon-based materials: a review

Kannapan Panchamoorthy Gopinath et al.

Summary: Carbon-based materials such as biochar, activated carbon, carbon nanotubes and graphene play a crucial role in environmental pollution control. They demonstrate high adsorption and removal efficiency for toxic gases and pollutants in air and water, while also significantly impacting biogas production and ammonia emissions.

ENVIRONMENTAL CHEMISTRY LETTERS (2021)

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Article Engineering, Environmental

Silver iodide decorated ZnSn(OH)6 hollow cube: Room-temperature preparation and application for highly efficient photocatalytic oxytetracycline degradation

Chen Zhang et al.

Summary: AgI/ZnSn(OH)(6) hollow cube nanocomposite was prepared to enhance visible-light-driven photocatalytic activity. The AgI/ZSH showed superior degradation effect for oxytetracycline hydrochloride (OTC) compared with AgI and ZnSn(OH)(6), and exhibited excellent performance in different environments without significant degradation after four cycles. The main active species were identified as superoxide radical and holes, and the degradation products and possible pathways of OTC were analyzed.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Engineering, Environmental

Catalyst bridging-mediated electron transfer for nonradical degradation of bisphenol A via natural manganese ore-cornstalk biochar composite activated peroxymonosulfate

Zhao Yang et al.

Summary: This study developed a novel PMS activator for water remediation, utilizing natural minerals and agricultural waste to prepare a composite catalyst for efficient and eco-friendly pollutant degradation. Experimental results demonstrate the excellent performance of the system in degrading pollutants, along with its high practical application potential.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Engineering, Environmental

Active MnO2/biochar composite for efficient As(III) removal: Insight into the mechanisms of redox transformation and adsorption

Dinh Viet Cuong et al.

Summary: An active MnO2/rice husk biochar composite (MBC) with improved porous structure was prepared for enhanced removal of As(III) in groundwater. MBC exhibited a high removal capacity for As(III) and a powerful transformation capability of As(III), with pH influencing its removal efficiency. MnO2 and the BC substrate played important roles in the effective removal of arsenic by MBC.

WATER RESEARCH (2021)

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Article Environmental Sciences

Preparation of ammonium-modified cassava waste-derived biochar and its evaluation for synergistic adsorption of ternary antibiotics from aqueous solution

Jiwei Luo et al.

Summary: The NH4+-modified biochar showed higher sorption affinity for norfloxacin (NOR) and sulfamerazine (SMR) compared to the raw biochar, while the raw biochar exhibited higher sorption affinity for oxytetracycline (OTC). OTC had the highest sorption to both biochars, followed by NOR and SMR. Additionally, electrostatic interactions among the ionic antibiotics in the multicomponent solution increased NOR and SMR sorption to both biochars.

JOURNAL OF ENVIRONMENTAL MANAGEMENT (2021)

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Article Environmental Sciences

Global evolution of research on green energy and environmental technologies:A bibliometric study

Hao Tan et al.

Summary: The study shows that publications on green energy and environmental technologies have grown exponentially, with China, the USA, and Italy being the most active countries, but global cooperation is not closely knit at present. The research frontier identification results indicate that categories such as energy, wastewater, and performance are stable, while catalyst and CO2 emission categories show a clear shift, suggesting that catalytic production of clean energy, strategies to reduce greenhouse gas emissions, and related studies are the research frontiers to address global energy crisis and environmental problems.

JOURNAL OF ENVIRONMENTAL MANAGEMENT (2021)

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Review Engineering, Environmental

Tuning oxygenated functional groups on biochar for water pollution control: A critical review

Lichun Dai et al.

Summary: Biochar has gained attention in water pollution control due to its tunable physico-chemical properties, especially the oxygenated functional groups (OFGs) which act as key active sites for pollutant removal through adsorption and redox reactions. Various strategies for tuning OFGs on biochar have been explored, such as in-situ and ex-situ oxidation, as well as grafting carboxyl groups via reactions like cycloaddition/acylation, leading to enhanced performance in pollutant removal.

JOURNAL OF HAZARDOUS MATERIALS (2021)

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Article Engineering, Environmental

Enhanced Oxidation of Organic Contaminants by Iron(II)-Activated Periodate: The Significance of High-Valent Iron-Oxo Species

Yang Zong et al.

Summary: Potassium periodate (PI, KIO4) can be activated by Fe(II) under acidic conditions to rapidly remove organic contaminants, generating high-valent iron-oxo species Fe(IV) and avoiding the formation of harmful iodine species. Isotope labeling techniques and X-ray absorption spectroscopy provided insights into the reaction mechanism of Fe(II)/PI process, enhancing our understanding of the efficient removal of emerging contaminants.

ENVIRONMENTAL SCIENCE & TECHNOLOGY (2021)

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Article Engineering, Chemical

Degradation of cephalexin by persulfate activated with magnetic loofah biochar: Performance and mechanism

Haocheng Song et al.

Summary: Antibiotic contamination is a serious environmental concern, and sulfate radical-based advanced oxidation processes have shown potential for treatment. A magnetic biochar derived from loofah was used to activate persulfate for cephalexin degradation, with the C-OH of the catalyst playing a crucial role. The conversion between Fe3+ and Fe2+ enhanced the degradation by producing SO4 center dot-, indicating broad adaptability and applications of the catalyst.

SEPARATION AND PURIFICATION TECHNOLOGY (2021)

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Article Engineering, Chemical

Study on the nonradical pathways of nitrogen-doped biochar activating persulfate for tetracycline degradation

Quanfa Zhong et al.

Summary: Nitrogen-doped biochar was successfully synthesized and used for degrading tetracycline, showing enhanced catalytic performance. The study provides an efficient and environmentally friendly method for antibiotic wastewater treatment.

SEPARATION AND PURIFICATION TECHNOLOGY (2021)

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Article Engineering, Environmental

Peroxymonosulfate/LaCoO3 system for tetracycline degradation: Performance and effects of co-existing inorganic anions and natural organic matter

Xue Yang et al.

Summary: The activation of peroxymonosulfate (PMS) by LaCoO3 is an efficient method for degrading tetracycline (TC) by generating reactive oxygen species (ROS). The presence of inorganic anions and low concentration of natural organic matter can enhance the degradation efficiency, while LaCoO3 shows stable reusability.

JOURNAL OF WATER PROCESS ENGINEERING (2021)

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Article Engineering, Environmental

Catalyst-free activation of permanganate under visible light irradiation for sulfamethazine degradation: Experiments and theoretical calculation

Chen Zhang et al.

Summary: This study utilized visible light to activate permanganate for the degradation of sulfamethazine, demonstrating the effective degradation of SMT in the VL/PM system. Factors influencing degradation and degradation mechanisms were investigated through experiments and Density Functional Theory calculations.

WATER RESEARCH (2021)

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Article Engineering, Environmental

Photocatalytic degradation of oxytetracycline under visible light by nanohybrids of CoFe alloy nanoparticles and nitrogen-/sulfur-codoped mesoporous carbon

Shuai Zhang et al.

Summary: Efficient photocatalysts CoFe@NSC were synthesized for enhanced degradation of oxytetracycline under visible light, showing promising potential for the development of novel catalysts for antibiotic photodegradation.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Environmental Sciences

Efficient degradation of diclofenac sodium by periodate activation using Fe/Cu bimetallic modified sewage sludge biochar/UV system

Liuyang He et al.

Summary: Iron/copper bimetallic nanoparticles based sludge biochar (Fe/Cu-SBC) was successfully prepared and applied for the activation of periodate to degrade diclofenac sodium. The catalytic efficiency of Fe/Cu-SBC system was improved under optimized conditions, showing great potential for the degradation of pharmaceuticals and personal care products (PPCPs) in wastewater.

SCIENCE OF THE TOTAL ENVIRONMENT (2021)

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Article Environmental Sciences

Goethite/biochar-activated peroxymonosulfate enhances tetracycline degradation: Inherent roles of radical and non-radical processes

Yanxiu Guo et al.

Summary: The study investigates the application of a novel goethite/biochar composite as an activator for tetracycline degradation in sulfate radical based AOPs. The catalytic efficiency of goethite/biochar is achieved through both radical and non-radical processes, with carbonyl group and Fe species identified as the main active sites. The study also proposes a reasonable degradation pathway for tetracycline based on the analysis of by-products and molecular structure.

SCIENCE OF THE TOTAL ENVIRONMENT (2021)

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Article Engineering, Environmental

The superior adsorption capacity of boron-nitrogen co-doping walnut shell biochar powder for Au(III), Pt(IV), and Pd(II)

Zejuan Wang et al.

Summary: Walnut shell biomass material, particularly the boron-nitrogen co-doped walnut shell biochar powder, has shown great potential in removing heavy metals through adsorption. Experimental results demonstrated high adsorption rates for Au(III), Pt(IV), and Pd(II), with adsorption kinetics following a quasi-two-stage model and isotherm equilibrium data aligning with the Langmuir isotherm model. The reaction mechanism between B-N-WSBP and noble metal ions was found to belong to chemical and single-layer adsorption.

JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING (2021)

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Article Engineering, Environmental

Surface construction of nitrogen-doped chitosan-derived carbon nanosheets with hierarchically porous structure for enhanced sulfacetamide degradation via peroxymonosulfate activation: Maneuverable porosity and active sites

Xiao Chen et al.

CHEMICAL ENGINEERING JOURNAL (2020)

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Article Engineering, Environmental

Role of radical and non-radical pathway in activating persulfate for degradation of p-nitrophenol by sulfur-doped ordered mesoporous carbon

Shiyu Liu et al.

CHEMICAL ENGINEERING JOURNAL (2020)

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Article Engineering, Environmental

Photocatalytic difference of amoxicillin and cefotaxime under visible light by mesoporous g-C3N4: Mechanism, degradation pathway and DFT calculation

Mengmeng Dou et al.

CHEMICAL ENGINEERING JOURNAL (2020)

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Article Environmental Sciences

Photocatalytic behavior of biochar-modified carbon nitride with enriched visible-light reactivity

Lirong Meng et al.

CHEMOSPHERE (2020)

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Review Environmental Sciences

Occurrence, formation, environmental fate and risks of environmentally persistent free radicals in biochars

Emmanuel Stephen Odinga et al.

ENVIRONMENT INTERNATIONAL (2020)

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Article Environmental Sciences

Manganese-modified biochar for highly efficient sorption of cadmium

Xiao Tan et al.

ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH (2020)

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Article Engineering, Environmental

Biochar-supported nanoscale zero-valent iron as an efficient catalyst for organic degradation in groundwater

Zhe Li et al.

JOURNAL OF HAZARDOUS MATERIALS (2020)

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Article Environmental Sciences

Fabrication of sustainable manganese ferrite modified biochar from vinasse for enhanced adsorption of fluoroquinolone antibiotics: Effects and mechanisms

Yujia Xiang et al.

SCIENCE OF THE TOTAL ENVIRONMENT (2020)

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Article Engineering, Environmental

Periodate activation with manganese oxides for sulfanilamide degradation

Jiangkun Du et al.

WATER RESEARCH (2020)

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Article Engineering, Environmental

Production of Reactive Oxygen Species by the Reaction of Periodate and Hydroxylamine for Rapid Removal of Organic Pollutants and Waterborne Bacteria

Hongwei Sun et al.

ENVIRONMENTAL SCIENCE & TECHNOLOGY (2020)

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Article Engineering, Environmental

Degradation of sulfamethazine by biochar-supported bimetallic oxide/persulfate system in natural water: Performance and reaction mechanism

Fanzhi Qin et al.

JOURNAL OF HAZARDOUS MATERIALS (2020)

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Article Chemistry, Physical

Molecular engineering of polymeric carbon nitride for highly efficient photocatalytic oxytetracycline degradation and H2O2 production

Yang Yang et al.

APPLIED CATALYSIS B-ENVIRONMENTAL (2020)

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Article Environmental Sciences

Singlet oxygen mediated the selective removal of oxytetracycline in C/Fe3C/Fe0 system as compared to chloramphenicol

Nan Zhao et al.

ENVIRONMENT INTERNATIONAL (2020)

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The antimony sorption and transport mechanisms in removal experiment by Mn-coated biochar

Xiaocen Jia et al.

SCIENCE OF THE TOTAL ENVIRONMENT (2020)

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Ferrous ion-tartaric acid chelation promoted calcium peroxide fenton-like reactions for simulated organic wastewater treatment

Shoufeng Tang et al.

JOURNAL OF CLEANER PRODUCTION (2020)

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Review Engineering, Environmental

Recent advances in application of graphitic carbon nitride-based catalysts for degrading organic contaminants in water through advanced oxidation processes beyond photocatalysis: A critical review

Yang Yang et al.

WATER RESEARCH (2020)

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Article Chemistry, Physical

Photo-Fenton degradation of emerging pollutants over Fe-POM nanoparticle/porous and ultrathin g-C3N4 nanosheet with rich nitrogen defect: Degradation mechanism, pathways, and products toxicity assessment

Jingjing Jiang et al.

APPLIED CATALYSIS B-ENVIRONMENTAL (2020)

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Impact of oxytetracycline on anaerobic wastewater treatment and mitigation using enhanced hydrolysis pretreatment

Yupeng He et al.

WATER RESEARCH (2020)

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Review Green & Sustainable Science & Technology

Critical Review on Biochar-Supported Catalysts for Pollutant Degradation and Sustainable Biorefinery

Manish Kumar et al.

ADVANCED SUSTAINABLE SYSTEMS (2020)

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Article Engineering, Environmental

New insights into the formation and transformation of active species in nZVI/BC activated persulfate in alkaline solutions

Haoyu Luo et al.

CHEMICAL ENGINEERING JOURNAL (2019)

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Article Chemistry, Physical

Insight into the energy band alignment of magnetically separable Ag2O/ZnFe2O4 p-n heterostructure with rapid charge transfer assisted visible light photocatalysis

Hai Guo et al.

JOURNAL OF CATALYSIS (2019)

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Article Chemistry, Physical

Boron nitride quantum dots decorated ultrathin porous g-C3N4: Intensified exciton dissociation and charge transfer for promoting visible-light-driven molecular oxygen activation

Yang Yang et al.

APPLIED CATALYSIS B-ENVIRONMENTAL (2019)

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Adsorption behavior of engineered carbons and carbon nanomaterials for metal endocrine disruptors: Experiments and theoretical calculation

Chen Zhang et al.

CHEMOSPHERE (2019)

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Driving forces and barriers in the removal of phosphorus from water using crop residue, wood and sewage sludge derived biochars

Patrick M. Melia et al.

SCIENCE OF THE TOTAL ENVIRONMENT (2019)

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Article Chemistry, Physical

Facile assembled biochar-based nanocomposite with improved graphitization for efficient photocatalytic activity driven by visible light

Shujing Ye et al.

APPLIED CATALYSIS B-ENVIRONMENTAL (2019)

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Insights into periodate oxidation of bisphenol A mediated by manganese

Jiangkun Du et al.

CHEMICAL ENGINEERING JOURNAL (2019)

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Review Engineering, Environmental

Biochar for environmental management: Mitigating greenhouse gas emissions, contaminant treatment, and potential negative impacts

Chen Zhang et al.

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Synthesis of MgO-coated corncob biochar and its application in lead stabilization in a soil washing residue

Zhengtao Shen et al.

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Investigating the adsorption behavior and the relative distribution of Cd2+ sorption mechanisms on biochars by different feedstock

Rong-Zhong Wang et al.

BIORESOURCE TECHNOLOGY (2018)

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Degradation kinetics and transformation products of chlorophene by aqueous permanganate

Xinxin Xu et al.

WATER RESEARCH (2018)

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Natural Fe-bearing manganese ore facilitating bioelectro-activation of peroxymonosulfate for bisphenol A oxidation

Suding Yan et al.

CHEMICAL ENGINEERING JOURNAL (2018)

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Effects of Peanut Shell Biochar on the Adsorption of Cd(II) by Paddy Soil

Chao Xu et al.

BULLETIN OF ENVIRONMENTAL CONTAMINATION AND TOXICOLOGY (2017)

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Enhanced adsorption of Cu(II) and Cd(II) by phosphoric acid-modified biochars

Hongbo Peng et al.

ENVIRONMENTAL POLLUTION (2017)

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Direct photolysis of oxytetracycline: Influence of initial concentration, pH and temperature

Xin Jin et al.

JOURNAL OF PHOTOCHEMISTRY AND PHOTOBIOLOGY A-CHEMISTRY (2017)

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Combination of Fenton processes and biotreatment for wastewater treatment and soil remediation

Danlian Huang et al.

SCIENCE OF THE TOTAL ENVIRONMENT (2017)

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Sorptive removal of ionizable antibiotic sulfamethazine from aqueous solution by graphene oxide-coated biochar nanocomposites: Influencing factors and mechanism

Danlian Huang et al.

CHEMOSPHERE (2017)

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Photogeneration of reactive oxygen species from biochar suspension for diethyl phthalate degradation

Guodong Fang et al.

APPLIED CATALYSIS B-ENVIRONMENTAL (2017)

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Visible-light-induced activation of periodate that mimics dye-sensitization of TiO2: Simultaneous decolorization of dyes and production of oxidizing radicals

Eun-Tae Yun et al.

APPLIED CATALYSIS B-ENVIRONMENTAL (2017)

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Lead and cadmium sorption mechanisms on magnetically modified biochars

Lukas Trakal et al.

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Efficient sonochemical degradation of perfluorooctanoic acid using periodate

Yu-Chi Lee et al.

ULTRASONICS SONOCHEMISTRY (2016)

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Efficacy of carbonaceous nanocomposites for sorbing ionizable antibiotic sulfamethazine from aqueous solution

Chen Zhang et al.

WATER RESEARCH (2016)

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Core-shell composite of wood-derived biochar supported MnO2 nanosheets for supercapacitor applications

Caichao Wan et al.

RSC ADVANCES (2016)

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Effect of temperature, pH and illumination on abiotic degradation of oxytetracycline in sterilized swine manure

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One-step synthesis of sea urchin-like α-MnO2 using KIO4 as the oxidant and its oxidation of arsenite

Mingxia Wang et al.

MATERIALS LETTERS (2012)

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Magnetite/graphene nanosheet composites: interfacial interaction and its impact on the durable high-rate performance in lithium-ion batteries

Jisheng Zhou et al.

RSC ADVANCES (2011)

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Photochemical decomposition of perfluorooctanoic acid in aqueous periodate with VUV and UV light irradiation

M. H. Cao et al.

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Pyrolitic carbon from biomass precursors as anode materials for lithium batteries

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MATERIALS SCIENCE AND ENGINEERING A-STRUCTURAL MATERIALS PROPERTIES MICROSTRUCTURE AND PROCESSING (2006)

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Kinetics and mechanism of photoactivated periodate reaction with 4-chlorophenol in acidic solution

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ENVIRONMENTAL SCIENCE & TECHNOLOGY (2004)

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Degradation of atrazine by manganese-catalysed ozonation - Influence of radical scavengers

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WATER RESEARCH (2000)

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Periodate activated by manganese oxide/biochar composites for antibiotic degradation in aqueous system: Combined effects of active manganese species and biochar

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