Journal
ENVIRONMENTAL MONITORING AND ASSESSMENT
Volume 194, Issue 6, Pages -Publisher
SPRINGER
DOI: 10.1007/s10661-022-10062-3
Keywords
Polycyclic aromatic hydrocarbon; Combustion device; Household combustion; Domestic air quality
Categories
Funding
- National Research Foundation of South Africa
- National Research Fund of Kenya [105807]
- Maasai Mara University, Kenya
- University of Pretoria, South Africa
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This study sampled gas phase emissions from cooking devices used in urban and rural households in Kenya to measure the concentrations of polycyclic aromatic hydrocarbons (PAHs). The results showed variations in PAH concentrations due to different fuel types, combustion devices, climate, and household characteristics. Wood combustion using the 3-stone device had the highest average PAH concentration. The findings highlight the importance of monitoring PAH emissions from these cooking devices and fuels for public health and pollution mitigation.
Traditional combustion devices and fuels such as charcoal, wood and biomass, are widely utilised in rural and urban households in Africa. Incomplete combustion can generate air pollutants which are of human toxicological importance, including polycyclic aromatic hydrocarbons (PAHs). In this study, portable multi-channel polydimethylsiloxane rubber traps were used to sample gas phase emissions from cooking devices used in urban and rural households in Bomet and Narok counties of Kenya. A wide range of total PAH concentrations was found in samples collected (0.82 - 173.69 mu g/m(3)), which could be attributed to the differences in fuel type, combustion device, climate, and nature of households. Wood combustion using the 3-stone device had the highest average total PAH concentration of similar to 71 mu g/m(3). Narok had higher indoor total gas phase PAH concentrations averaging 35.88 mu g/m(3) in urban and 70.84 mu g/m(3) in rural households, compared to Bomet county (2.91 mu g/m(3) in urban and 9.09 mu g/m(3) in rural households). Ambient total gas phase PAH concentrations were more similar (Narok: 1.26 - 6.28 mu g/m(3) and Bomet: 2.44 - 6.30 mu g/m(3)). Although the 3-stone device and burning of wood accounted for higher PAH emissions, the charcoal burning jiko stove produced the highest toxic equivalence quotient. Monitoring of PAHs emitted by these cooking devices and fuels is critical to public health and sustainable pollution mitigation.
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