Journal
CRYSTAL GROWTH & DESIGN
Volume 22, Issue 4, Pages 2594-2601Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.cgd.2c00058
Keywords
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Funding
- Science Challenge Project [TZ2018004]
- National Natural Science Foundation of China [21875110, 22075143, 22105187]
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This study demonstrated a series of energetic compounds featuring intramolecular hydrogen bonds, with compound 6 identified as an ideal insensitive HEDM candidate due to its high density, good detonation properties, simple preparation, good thermostability, and insensitivity.
In this study, a series of energetic compounds featuring intramolecular hydrogen bonds were demonstrated by the substituted reaction with 5-aminotetrazole. Notably, the representative energetic compounds 3 and 6 exhibit high density (1.910 g cm(-3) and 1.905 g cm(-3)) and good detonation properties (3: D = 9072 m s-1, P = 37.1 GPa, 6: D = 8861 m s(-1), P = 32.3 GPa). Additionally, combining a series of other advantages such as simple preparation, good thermostability (T-d = 265 degrees C), and insensitivity (IS > 40 J, FS > 360 N), compound 6 is an ideal insensitive HEDM candidate.
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