Journal
CHEMISTRY-AN ASIAN JOURNAL
Volume 17, Issue 15, Pages -Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/asia.202200340
Keywords
Aromaticity; BN doping; Dual emission; Lewis acidity; Polycyclic aromatic hydrocarbons
Categories
Funding
- National Natural Science Foundation of China [22001135, 22109111]
- Education Department of Inner Mongolia Antonomous Region [NJYT22098]
- Natural Science Foundation of Zhejiang Province [LQ22B030006]
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A B-N embedded nitrogen-annulated perylene with unique properties has been successfully synthesized, which is isoelectronic to coronene but owns a five-membered pyrrole ring.
A B-N embedded nitrogen-annulated perylene has been successfully synthesized. The resultant molecule BN-NP is isoelectronic to coronene, but owns a five-membered pyrrole ring. Experiments and DFT calculations indicated that peripheral pyrrole and BN modifications endow BN-NP with various unique properties like bent structure, dual emission, efficient Lewis acidic response, peripheral aromaticity, narrowest energy band gap among all coronene isoelectronic structures and so on.
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