Journal
CHEMICAL ENGINEERING JOURNAL
Volume 431, Issue -, Pages -Publisher
ELSEVIER SCIENCE SA
DOI: 10.1016/j.cej.2021.134284
Keywords
Undaria pinnatifida; Superb electromagnetic wave absorption; Porous structure; Sustainable and low-cost
Categories
Funding
- National Natural Science of China [51971162, U1933112, 51671146]
- National Key Research and Development Program of China [2019YFE0122900]
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This study successfully fabricates spherical MoS2 nanoflowers/undaria pinnatifida-derived honeycomb-like porous carbon composites, which are easy to prepare, sustainable, and low-cost electromagnetic absorbing materials with super absorption capacity. The unique microstructure and porosity of the composites facilitate multiple scattering and reflections, as well as the construction of interconnected conducting networks, greatly enhancing the electromagnetic wave absorption capacity. These hybrids have potential applications as sustainable electromagnetic wave absorbers.
The increasingly serious electromagnetic pollution has caused an urgent demand for easy preparation, sustain-able and low-cost electromagnetic absorbing materials with super absorption capacity. Herein, inspired by the nature, spherical MoS2 nanoflowers/undaria pinnatifida-derived honeycomb-like porous carbon composites were fabricated by a simple carbonization and subsequent hydrothermal process. The unique honeycomb-like porous microstructure of undaria pinnatifida facilitates the generation of multiple scattering and reflections and the construction of interconnected conducting networks, while the rich porous structure provides a vast surface for the growth of MoS2 crystals. In addition, MoS2 significantly not only improved the impedance matching of the composites but also greatly enhanced the polarization loss due to the simultaneous growth of MoS2 nanoflowers on the surface and in the internal pores of the undaria pinnatifida. As a result, the hybrids achieved a maximum electromagnetic wave (EMW) absorption capacity with a reflection loss (RL) value of up to-75.94 dB at a thickness of only 1.68 mm. The results indicated that the C/MoS2 hybrids can be a new prospective candidate as sustainable EMW absorbers with low density and superb EMW absorption performance.
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