4.7 Article

Airborne measurements of cloud condensation nuclei (CCN) vertical structures over Southern China

Journal

ATMOSPHERIC RESEARCH
Volume 268, Issue -, Pages -

Publisher

ELSEVIER SCIENCE INC
DOI: 10.1016/j.atmosres.2021.106012

Keywords

Cloud condensation nuclei ( CCN ); Airborne in-situ measurement; CCN vertical structure, CCN spectrum

Funding

  1. National Natural Science Foundation of China [41822504, 42075083]
  2. National Key Research and Development Program of China [2017YFC1501806]
  3. Basic Research Fund of Chinese Academy of Meteorological Sciences [2021Y028]

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This study investigates the vertical structures of cloud condensation nuclei (CCN) over southern China and finds that CCN concentration peaks near 1.3 km above the ground and then sharply decreases above 2.5 km. A segmentation fitting approach is used to describe the CCN structure, and the CCN particle size distribution changes with increasing water vapor supersaturation. The results provide insight for cloud microphysical parameterization in numerical models and weather modification.
In this study, the vertical structures of cloud condensation nuclei (CCN) over southern China are investigated with two flight datasets during the period of 16-17 July 2019. The results show that the CCN number con-centration (N-CCN) increases first with the increasing height, peaking near 1.3 km above the ground, and then decreases sharply to a low value above 2.5 km. Good agreement is obtained by employing a segmentation fitting approach to describe the vertical CCN structure. More specifically a simple linear function is used to fit the N-CCN below 1.3 km; a polynomial function is utilized to describe the measurements between 1.3 km and 2.5 km, and, a constant value of 7 cm(-3) is assigned above 2.5 km. The CCN particle size distribution (CPSD) presents a unimodal mode with the peak that changes to the direction of larger diameter with growing water vapor supersaturation (SS). As for the effects of SS, N-CCN, as well as the diameter of CCN increases with the increasing SS. The CCN spectrum is well represented by the classical Twomey power-law function of N-CCN(SS) = C.SSk. Although the values of parameter C are 72 cm(-3) and 150 cm(-3) in the two measurements, respectively, the paramer k changes a little with its values being 1.5 or so. The results gained herein might be helpful for cloud microphysical parameterization in numerical models and provide a guide for weather modification.

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