Journal
APPLIED RADIATION AND ISOTOPES
Volume 181, Issue -, Pages -Publisher
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.apradiso.2022.110105
Keywords
Dosimetry; Electron spin resonance; New dosimeters; Lithium; Potassium; Sodium
Categories
Funding
- Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP) [2013/03258-9, 2007/06720-4, 2013/07699-0]
- Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq) [304107/2019-0, 309186/2020-0]
Ask authors/readers for more resources
This study presents the first investigation of materials for ESR dosimetry, emphasizing on radiological characteristics, dose sensitivity, and signal stability. Among the analyzed compounds, sodium citrate shows promising characteristics as a dosimeter material.
This work consists of a first investigation of materials that could be used as ESR dosimeters with doses up to 5 Gy aiming possible applications that would include retrospective dosimetry or dosimetry in specific applications. The characteristics considered were radiological properties close to that of soft tissues, evaluated through their effective atomic number and mass attenuation coefficient, ESR signal dependence on the irradiation dose, sensitivity to dose in the range of-5 Gy when exposed to a 50 kV x-ray source and signal stability over a 30-day period. A total of 16 compounds of lithium, potassium and sodium were analyzed, including the already known dosimeter material, lithium formate. Among them, lithium carbonate, lithium phosphate, sodium formate, so-dium acetate, sodium citrate, sodium dithionite, sodium carbonate, showed eligible characteristics. After analyzing the ESR dose-response curves, the molecules that showed greater sensitivity to radiation in descending order are: sodium formate, sodium acetate, sodium citrate and sodium dithionite, however, lower than lithium formate. Sodium formate and sodium citrate presented ESR signals with high stability, similar to lithium formate, with fading of-3% in 30 days, different from sodium acetate, which showed a 19% reduction. Sodium citrate also presents radiological properties close to soft tissue. Therefore, considering all properties, in the set of the new materials studied in this work, sodium citrate is a promising material for ESR dosimetry.
Authors
I am an author on this paper
Click your name to claim this paper and add it to your profile.
Reviews
Recommended
No Data Available