Journal
AICHE JOURNAL
Volume 68, Issue 9, Pages -Publisher
WILEY
DOI: 10.1002/aic.17761
Keywords
1DMA2P; ANN models; CO2 loading; empirical model; physical properties
Categories
Funding
- Natural Science and Engineering Research Council of Canada (NSERC)
- talent project from Beijing Institute of Technology [2022CX01004]
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This work investigates the thermophysical properties of pure 1-dimethylamino-2-propanol (1DMA2P) and its aqueous solutions with CO2 loading. The density, viscosity, and specific heat capacity were measured over a range of concentrations and temperatures. Both empirical models and artificial neural network (ANN) models were used to correlate the experimental results, with the ANN models showing better prediction accuracy. This study provides a potential method for predicting the physical properties of aqueous amine CO2 absorption systems.
In this work, the density, viscosity, and specific heat capacity of pure 1-dimethylamino-2-propanol (1DMA2P) as well as aqueous unloaded and CO2-loaded 1DMA2P solution (with a CO2 loading of 0.04-0.70 mol CO2/mol amine) were measured over the 1DMA2P concentration range of 0.5-3.0 mol/L and temperature range of 293-323 K. The observed experimental results of these thermophysical properties of the 1DMA2P-H2O-CO2 system were correlated using empirical models as well as artificial neural network (ANN) models (namely, back-propagation neural network [BPNN] and radial basis function neural network [RBFNN] models). It was found that the developed BPNN and RBFNN models could predict the experimental results of 1DMA2P-H2O-CO2 better than correlations using empirical models. The results could be treated as one of the accurate and potential methods to predict the physical properties for aqueous amine CO2 absorption systems.
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