Journal
ACS NANO
Volume 16, Issue 5, Pages 8128-8140Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acsnano.2c01455
Keywords
GaSb; nanowire arrays; sulfur-passivation; polarized photodetector; imaging sensor
Categories
Funding
- Postdoctoral Science Foundation of China [2021M703458]
- National Natural Science Foundation of China [62125404]
- Strategic Priority Research Program of Chinese Academy of Sciences [XDB43000000]
- Natural Science Foundation of Hebei Province [E2021201043]
- Hundred Talents Plan of Hebei Province [E2018100001]
- Research Grants Council of the Hong Kong Special Administrative Region, China [CityU RFS2021-1S04]
- City University of Hong Kong [7005236]
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The near-infrared polarimetric image sensor has become a research hotspot due to its wide range of applications. The ordered GaSb nanowire arrays synthesized through a sulfur-catalyzed chemical vapor deposition process show potential for near-infrared polarization photodetection. The sulfur-passivation GaSb nanowire-based photodetector exhibits lower dark current and higher responsivity than pure GaSb nanowires. A flexible polarimetric image sensor with good imaging ability for incident near-infrared polarization light is successfully constructed on the ordered S-GaSb nanowire arrays. These properties empower ordered S-GaSb nanowire arrays with technological potentials in next-generation large-scale near-infrared polarimetric imaging sensors.
The near-infrared polarimetric image sensor has a wide range of applications in the military and civilian fields, thus developing into a research hotspot in recent years. Because of their distinguishing ID structure features, the ordered GaSb nanowire (NW) arrays possess potential applications for near-infrared polarization photodetection. In this work, single-crystalline GaSb NWs are synthesized through a sulfurcatalyzed chemical vapor deposition process. A sulfur-passivation thin layer is formed on the NW surface, which prevents the GaSb NW core from being oxidized. The photodetector based on sulfur-passivation GaSb (S-GaSb) NWs has a lower dark current and higher responsivity than that built with pure GaSb NWs. The photodetector exhibits a large responsivity of 9.39 X 10(2) A/W and an ultrahigh detectivity of 1.10 x 10(11) Jones for 1.55 mu m incident light. Furthermore, the dichroic ratio of the device is measured to reach 2.65 for polarized 1.55 mu m light. Through a COMSOL simulation, it is elucidated that the origin of the polarized photoresponse is the attenuation of a light electric field inside the NW when the angle of incident polarization light rotates. Moreover, a flexible polarimetric image sensor with 5 X 5 pixels is successfully constructed on the ordered S-GaSb NW arrays, and it exhibits a good imaging ability for incident near-infrared polarization light. These good photoresponse properties and polarized imaging abilities can empower ordered S-GaSb NW arrays with technological potentials in next-generation large-scale near-infrared polarimetric imaging sensors.
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