4.8 Review

Toward Continuous-Wave Pumped Metal Halide Perovskite Lasers: Strategies and Challenges

Journal

ACS NANO
Volume 16, Issue 5, Pages 7116-7143

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acsnano.1c11539

Keywords

metal halide perovskites; continuous-wave lasers; thermal management; cavity engineering; quantum-well-like structure; triplet states; lasing death; photophysics

Funding

  1. National Key Research and Development Program of China [2021YFA1401100]
  2. Fundamental Research Funds for the Central Universities [ZYGX2019Z018]
  3. Innovation Group Project of Sichuan Province [20CXTD0090]
  4. UESTC Shared Research Facilities of Electromagnetic Wave and Matter Interaction [Y0301901290100201]

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This review discusses the challenges and opportunities in improving the performance and stability of continuous-wave (CW) pumped perovskite lasers. Potential strategies from material to device levels are examined, and future prospects are proposed.
Reliable and efficient continuous-wave (CW) lasers have been intensively pursued in the field of optoelectronic integrated circuits. Metal perovskites have emerged as promising gain materials for solution-processed laser diodes. Recently, the performance of CW perovskite lasers has been improved with the optimization of material and device levels. Nevertheless, the realization of CW pumped perovskite lasers is still hampered by thermal runaway, unwanted parasitic species, and poor long-term stability. This review starts with the charge carrier recombination dynamics and fundamentals of CW lasing in perovskites. We examine the potential strategies that can be used to improve the performance of perovskite CW lasers from the materials to device levels. We also propose the open challenges and future opportunities in developing highperformance and stable CW pumped perovskite lasers.

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