4.8 Article

Active and Smart Terahertz Electro-Optic Modulator Based on VO2 Structure

Journal

ACS APPLIED MATERIALS & INTERFACES
Volume 14, Issue 23, Pages 26923-26930

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acsami.2c04736

Keywords

electro-optic modulation; THz modulation; antireflection; VO2 thin film; smart control

Funding

  1. National Key R&D Program of China [2021YFA1600200, 2017YFA0303603]
  2. National Natural Science Foundation of China [U2032218, 12111530283, 61805256]
  3. Plan for Major Provincial Science & Technology Project [202003a05020018]
  4. Key Research Program of Frontier Sciences, CAS [QYZDB-SSW-SLH011]
  5. Users with Excellence Program of Hefei Science Center CAS [2021HSCUE009]
  6. High Magnetic Field Laboratory of Anhui Province

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This article demonstrates an active and smart electro-optic terahertz modulator based on strongly correlated electron oxide vanadium dioxide. By applying an external electric field, the transmission, reflection, absorption, and phase of terahertz waves can be efficiently modulated, with the ability to stabilize the antireflection condition.
Modulating terahertz (THz) waves actively and smartly through an external field is highly desired in the development of THz spectroscopic devices. Here, we demonstrate an active and smart electro-optic THz modulator based on a strongly correlated electron oxide vanadium dioxide (VO2). With milliampere current excitation on the VO2 thin film, the transmission, reflection, absorption, and phase of THz waves can be modulated efficiently. In particular, the antireflection condition can be actively achieved and the modulation depth reaches 99.9%, accompanied by a 180 degrees phase switching. Repeated and current scanning experiments confirm the high stability and multibit modulation of this electro-optic modulation. Most strikingly, by utilizing a feedback loop of THz-electro-THz geometry, a smart electro-optic THz control is realized. For instance, the antireflection condition can be stabilized precisely no matter what the initial condition is and how the external environment changes. The proposed electro-optic THz modulation method, taking advantage of strongly correlated electron material, opens up avenues for the realization of THz smart devices.

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