4.7 Article

SnSe Nanoplates for Photodetectors with a High Signal/Noise Ratio

Journal

ACS APPLIED NANO MATERIALS
Volume 4, Issue 12, Pages 13071-13078

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acsanm.1c02595

Keywords

SnSe nanoplates; semiconductors; 2D nanomaterials; CVD growth; photoconductor detectors; high signal/noise ratio

Funding

  1. Australian Research Council [DP200103188, LE200100032, DP170104562, LP170100088, LE170100233, FT130101708]
  2. UWA Research Impact Grant
  3. Australian Research Council [LE200100032, DP200103188] Funding Source: Australian Research Council

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This work reported a study on two-dimensional SnSe nanoplates grown by chemical vapor deposition and their applications in single nanoplate photodetectors. The SnSe nanoplates exhibited excellent device performance with high responsivity, specific detectivity, and external quantum efficiency, as well as low dark current and white noise, resulting in a high signal-to-noise ratio for the detector device.
In this work, we report a study on two-dimensional SnSe nanoplates grown by chemical vapor deposition and their applications in single nanoplate photodetectors with a high signal/noise ratio. The SnSe nanoplates present a square shape with a lateral size (side length) up to similar to 8 mu m. The lateral dimension of SnSe nanoplates increases with increasing the growth temperature from 400 to 440 degrees C and then saturates with increasing the growth temperature further due to the competition between SnSe molecules transported and those consumed on the surface of the substrate. The SnSe nanoplate photodetectors fabricated show excellent device performance at room temperature with a responsivity of 1.32 A/W, a specific detectivity of 1.01 X 10(11) Jones, an external quantum efficiency of 408.37%, and a response time (t(rising)/t(reset)) of 0.24/0.15 s under 1 V bias and 400 nm laser illumination. More importantly, the SnSe nanoplate photodetector exhibits a dark current of 130 pA, a low white noise of 4.8 x 10(-15)A/Hz(1/2), and a high photo-switching ratio up to 176.14, which is the highest value reported so far for a SnSe photodetector. The low-level dark current and white noise indicate a high signal-to-noise ratio for the SnSe nanoplate detector device. These detector performance parameters imply the great promise of SnSe nanoplates for applications in making photodetectors with low noise and a high signal/noise ratio.

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