Journal
CANADIAN JOURNAL OF CHEMISTRY
Volume 93, Issue 8, Pages 882-887Publisher
CANADIAN SCIENCE PUBLISHING, NRC RESEARCH PRESS
DOI: 10.1139/cjc-2014-0507
Keywords
methane hydrate; nucleation rate; induction time; crude oil; emulsion
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Nucleation of methane hydrate from water emulsions in five different kinds of crude oil and in decane have been studied with the use of isothermal methods. The experiments were conducted at a temperature of -5 degrees C and pressure of 12 MPa. It is shown that the nucleation rates tend to decrease with the increase in the density of the organic liquid used to make the emulsion. It is most likely that the observed regularities are related to the rate of methane diffusion to water surface.
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