Journal
ORGANIC CHEMISTRY FRONTIERS
Volume 9, Issue 7, Pages 1850-1854Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/d1qo01733k
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Funding
- National Natural Science Foundation of China [21901233]
- Natural Science Foundation of Zhejiang Province [LY21B020005]
- Open Research Fund of Key Laboratory of the Ministry of Education for Advanced Catalysis Materials, Zhejiang Normal University [KLMEACM201908]
- Zhejiang Key Laboratory for Reactive Chemistry on Solid Surfaces, Zhejiang Normal University [KLMEACM201908]
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A novel catalyst-controlled reaction is reported, which allows for the rapid and efficient synthesis of a series of bicyclic compounds by using readily available acyclic enyne-amides and crotonate-derived sulfur ylides as substrates.
A novel catalyst-controlled cycloisomerization/[4 + 3]cycloaddition sequence of readily available acyclic enyne-amides and crotonate-derived sulfur ylides is reported. This strategy enables the rapid and efficient construction of a series of bicyclic 2,3-furan-fused dihydroazepines and 2,3-pyrrole-fused dihydrooxepines with diverse substituents in generally good yield.
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