Ferromagnetic Double Perovskite Semiconductors with Tunable Properties

The authors successfully dope the magnetically silent double perovskite semiconductor Sr2GaSbO6 to induce ferromagnetism and tune its bandgap, with Ga3+ partially substituted by the magnetic trivalent cation Mn3+, in a rigid cation ordering with Sb5+. The new ferromagnetic semiconducting Sr2Ga1-xMnxSbO6 double perovskite, which crystallizes in tetragonal symmetry (space group I4/m) and has tunable ferromagnetic ordering temperature and bandgap, suggests that magnetic ion doping of double perovskites is a productive avenue toward obtaining materials for application in next-generation oxide-based spintronic devices.

Automated summary

The authors successfully doped Sr2GaSbO6, a magnetically silent double perovskite semiconductor, with magnetic trivalent cation Mn3+ to induce ferromagnetism and tune its bandgap. The new material, Sr2Ga1-xMnxSbO6 double perovskite, exhibits tunable ferromagnetic ordering temperature and bandgap, suggesting its potential application in next-generation oxide-based spintronic devices.