4.7 Article

Modelling of Environmental Ageing of Polymers and Polymer Composites-Modular and Multiscale Methods

Journal

POLYMERS
Volume 14, Issue 1, Pages -

Publisher

MDPI
DOI: 10.3390/polym14010216

Keywords

polymer; fibre; composite; biodegradable; environmental ageing; durability; modelling; mathematical modelling; multiscale modelling; diffusion; accelerated testing; lifetime prediction

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This paper summarizes the modelling methods for environmental ageing of polymers and polymer composites, including modular and multiscale approaches. These methods can predict the environmental ageing and degradation of materials, providing a deeper and reliable understanding, and enhancing confidence in the prediction of material's environmental durability.
Service lifetimes of polymers and polymer composites are impacted by environmental ageing. The validation of new composites and their environmental durability involves costly testing programs, thus calling for more affordable and safe alternatives, and modelling is seen as such an alternative. The state-of-the-art models are systematized in this work. The review offers a comprehensive overview of the modular and multiscale modelling approaches. These approaches provide means to predict the environmental ageing and degradation of polymers and polymer composites. Furthermore, the systematization of methods and models presented herein leads to a deeper and reliable understanding of the physical and chemical principles of environmental ageing. As a result, it provides better confidence in the modelling methods for predicting the environmental durability of polymeric materials and fibre-reinforced composites.

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