4.6 Article

In situ construction of a Te/CsPbBr3 heterojunction for self-powered photodetector

Journal

RSC ADVANCES
Volume 12, Issue 5, Pages 2729-2735

Publisher

ROYAL SOC CHEMISTRY
DOI: 10.1039/d1ra08236a

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Funding

  1. National Natural Science Foundation of China [61704012]
  2. Natural Science Foundation of Jiangsu Province of China [BK20191025]

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In this study, high-performance Te/CsPbBr3 photodetector was constructed by using CsPbBr3 particles prepared through a simple solvent evaporation method. The Te/CsPbBr3 photodetector exhibited improved photocurrent, excellent self-powered performance, broad-spectrum response, and ultra-fast response speed.
In this study, CsPbBr3 particles were prepared by a simple solvent evaporation method in ambient environment; the p-n heterojunction formed by CsPbBr3 particles on the surface of a single long Te wire was used to construct a high-performance Te/CsPbBr3 photodetector. Compared with CsPbBr3 PDs, the Te/CsPbBr3 photodetector showed improved photocurrent, and exhibited characteristics of excellent self-powered performance, broad-spectrum response (UV-visible), and ultra-fast response speed (t(rise) = 0.09 ms). In addition, under zero bias and upon 540 nm light irradiation, the device had good responsivity (0.35 mA W-1), high photosensitivity (up to 100 on/off ratio), and a detectivity of 1.42 x 10(10) Jones. This study provides insight into the possibility of manufacturing high-performance self-powered photodetectors through a simple in situ construction of heterojunctions.

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