Journal
NATURE COMMUNICATIONS
Volume 12, Issue 1, Pages -Publisher
NATURE PORTFOLIO
DOI: 10.1038/s41467-021-27218-3
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Funding
- National Natural Science Foundation of China [61761166009, 11974422, 61521004, 61874003, 62174005]
- Strategic Priority Research Program of the Chinese Academy of Sciences [XDB30000000]
- Elemental Strategy Initiative
- CREST [JPMJCR15F3]
- JST
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This study develops light helicity detectors based on graphene-Crl(3)-graphene hetero-structures, revealing the interplay between magnetic and optoelectronic properties in Crl(3) and paving the way for the development of spin-optoelectronic devices in the future.
Two-dimensional magnetic semiconductors provide a platform for studying physical phenomena at atomically thin limit, and promise magneto-optoelectronic devices application. Here, we report light helicity detectors based on graphene-Crl(3)-graphene vdW hetero-structures. We investigate the circularly polarized light excited current and reflective magnetic circular dichroism (RMCD) under various magnetic fields in both monolayer and multilayer Crl(3) devices. The devices exhibit clear helicity-selective photoresponse behavior determined by the magnetic state of Crl(3). We also find abnormal negative photocurrents at higher bias in both monolayer and multilayer Crl(3). A possible explanation is proposed for this phenomenon. Our work reveals the interplay between magnetic and optoelectronic properties in Crl(3) and paves the way to developing spin-optoelectronic devices.
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