4.8 Article

Compound jetting from bubble bursting at an air-oil-water interface

Journal

NATURE COMMUNICATIONS
Volume 12, Issue 1, Pages -

Publisher

NATURE PORTFOLIO
DOI: 10.1038/s41467-021-26382-w

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The study investigates the dynamics of bubble-bursting jets on oil-covered aqueous surfaces, demonstrating how this process can disperse insoluble organic contaminants. It advances the understanding of bubble bursting dynamics and may provide insights into the airborne transmission of organic matters related to aerosol production in nature.
How structurally complex interfaces mediate bubble bursting might significantly impact environmental and industrial processes. Here, authors investigate the bubble-bursting jets dynamics of oil-covered aqueous surface and show how these can also disperse insoluble organic contaminants. Bursting of bubbles at a liquid surface is ubiquitous in a wide range of physical, biological, and geological phenomena, as a key source of aerosol droplets for mass transport across the interface. However, how a structurally complex interface, widely present in nature, mediates the bursting process remains largely unknown. Here, we document the bubble-bursting jet dynamics at an oil-covered aqueous surface, which typifies the sea surface microlayer as well as an oil spill on the ocean. The jet tip radius and velocity are altered with even a thin oil layer, and oily aerosol droplets are produced. We provide evidence that the coupling of oil spreading and cavity collapse dynamics results in a multi-phase jet and the follow-up droplet size change. The oil spreading influences the effective viscous damping, and scaling laws are proposed to quantify the jetting dynamics. Our study not only advances the fundamental understanding of bubble bursting dynamics, but also may shed light on the airborne transmission of organic matters in nature related to aerosol production.

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