4.4 Article

Tailoring linear and nonlinear surface plasmon responses in borophene nanostructures

Journal

JOURNAL OF OPTICS
Volume 24, Issue 11, Pages -

Publisher

IOP Publishing Ltd
DOI: 10.1088/2040-8986/ac3eb1

Keywords

surface plasmon; dipole moment; second-order nonlinearity; lifetime

Categories

Funding

  1. Province Natural Science Foundation of Guangdong [2018A030313684]
  2. Guangdong Basic and Applied Basic Research Foundation [2020A1515110488]
  3. Scientific Key Research Fund of Guangdong Provincial Education Department [2019KZDXM061, 2019KQNCX099, 2020ZDZX2059]

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Borophene, a novel 2D material, shows significant influence in nanoscale materials and devices through its electric dipole transient and nonlinear effects. The scattering properties, lifetime evolution, and plasmonic modes can be controlled by tuning the carrier relaxation time, effective electron mass, and free carrier density, making it an excellent platform for tunable plasmonic-photonic devices.
The newly reported 2D material 'borophene' provides a novel building block for nanoscale materials and devices. In this work, the linear and nonlinear plasmonic response of the electric dipole (ED) moment in metallic borophene is theoretically investigated. In our proposed model, a borophene nanostructure is deposited on the top of a dielectric layer sandwich with a silver layer acting as a mirror. It was found that the scattering at the scattering peak originates mainly from the exciting total ED. Our calculations demonstrate that scattering in the proposed model can be tuned well with carrier relaxation time, effective electron mass and free carrier density. The strongly localized fundamental field induces the desired increase in the second harmonic wave, which is discussed in detail by introducing the second-order nonlinear source. In addition, the evolution of the lifetime of linear and nonlinear plasmonic modes is also investigated, which helps us to study the underlying mechanism of microprocessing in the borophene plasmonic-photonic interaction. The manipulation of plasmonic behaviour and lifetime evolution makes borophene an excellent platform for tunable plasmonic-photonic devices.

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