4.8 Review

Colloquium: Nonthermal pathways to ultrafast control in quantum materials

Journal

REVIEWS OF MODERN PHYSICS
Volume 93, Issue 4, Pages -

Publisher

AMER PHYSICAL SOC
DOI: 10.1103/RevModPhys.93.041002

Keywords

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Funding

  1. Max Planck-New York City Center forNon-Equilibrium Quantum Phenomena
  2. Deutsche Forschungsgemeinschaft (DFG, German Research Foundation) [EXC 2004/1-390534769]
  3. University of Pennsylvania
  4. Flatiron Institute
  5. Simons Foundation
  6. Cluster of Excellence CUI: Advanced Imaging of Matter of the DFG [390715994]
  7. DFG, SFB-925 [170620586]
  8. DFG via the Emmy Noether Program [SE 2558/2]

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Recent progress in utilizing ultrafast light-matter interaction to control the macroscopic properties of quantum materials is reviewed, focusing on photoinduced phenomena that are nonthermal in nature. These phenomena involve transient modifications to the free energy landscape, redistribution of quasiparticle populations, modification of coupling strengths, resonant driving of the crystal lattice, and coherent dressing of a material's quantum states by the light field. Discussing recently discovered effects leveraging these mechanisms and presenting a road map for utilizing nonthermal pathways to create new functionalities.
Recent progress in utilizing ultrafast light-matter interaction to control the macroscopic properties of quantum materials is reviewed. Particular emphasis is placed on photoinduced phenomena that do not result from ultrafast heating effects but rather emerge from microscopic processes that are inherently nonthermal in nature. Many of these processes can be described as transient modifications to the free energy landscape resulting from the redistribution of quasiparticle populations, the dynamical modification of coupling strengths, and the resonant driving of the crystal lattice. Other pathways result from the coherent dressing of a material's quantum states by the light field. A selection of recently discovered effects leveraging these mechanisms, as well as the technological advances that led to their discovery, is discussed. A road map for how the field can harness these nonthermal pathways to create new functionalities is presented.

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