4.8 Article

Topological liquid crystal superstructures as structured light lasers

Publisher

NATL ACAD SCIENCES
DOI: 10.1073/pnas.2110839118

Keywords

liquid crystals; topological structures; microlaser; vector beams

Funding

  1. Slovenian Research Agency [P1-0099, N2-0085, N1-0104, J1-1697, N1-0116]
  2. European Research Council under the European Union's Horizon 2020 research and innovation program [884928-LOGOS, 851143-CellLasers]

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Liquid crystals can form a variety of self-assembled topological structures with applications in optical and photonic devices, exhibiting unique properties such as self-assembly, self-healing, large tunability, sensitivity to external stimuli, and biocompatibility. By inserting topological defects into LC superstructures, complex tunable microlasers emitting structured light can be generated, with the topology and geometry of the LC superstructure determining the structuring of the emitted light.
Liquid crystals (LCs) form an extremely rich range of self-assembled topological structures with artificially or naturally created topological defects. Some of the main applications of LCs are various optical and photonic devices, where compared to their solid-state counterparts, soft photonic systems are fundamentally different in terms of unique properties such as self-assembly, self-healing, large tunability, sensitivity to external stimuli, and biocompatibility. Here we show that complex tunable microlasers emitting structured light can be generated from self-assembled topological LC superstructures containing topological defects inserted into a thin Fabry-Perot microcavity. The topology and geometry of the LC superstructure determine the structuring of the emitted light by providing complex three-dimensionally varying optical axis and order parameter singularities, also affecting the topology of the light polarization. The microlaser can be switched between modes by an electric field, and its wavelength can be tuned with temperature. The proposed soft matter microlaser approach opens directions in soft matter photonics research, where structured light with specifically tailored intensity and polarization fields could be designed and implemented.

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