4.8 Article

Band-selective gap opening by a C4-symmetric order in a proximity-coupled heterostructure Sr2VO3FeAs

Publisher

NATL ACAD SCIENCES
DOI: 10.1073/pnas.2105190118

Keywords

strong electron correlation; heterostructure; proximity coupling; iron-based superconductors

Funding

  1. National Research Foundation of Korea (NRF) [2015M3D1A1070672, 2020K1A3A7A09080366, 2020R1A4A2002828, 2021R1A2C1013119, 2019R1A6A1A10073887, 2019M3E4A1080411, 2020R1A4A3079707, 2021R1A2C4001847]
  2. Institute for Basic Science (IBS) through the Center for Artificial Low Dimensional Electronic System [IBS-R014-D1]
  3. NRF through Science Research Center (SRC) [2018R1A5A6075964]
  4. Max Planck-POSTECH Center for Complex Phase Materials [2016K1A4A4A01922028]
  5. research program of the IBS [IBS-R009-G2]
  6. Hochfeld-Magnetlabor Dresden
  7. Office of Basic Energy Science of the US Department of Energy [DE-AC02-05CH11231]
  8. National Research Foundation of Korea [2020R1A4A3079707, 2020K1A3A7A09080366, 2021R1A2C1013119, 2021R1A2C4001847, 2015M3D1A1070672] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)

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The unconventional gap opening in a hetero-structured iron-based superconductor Sr2VO3FeAs across a phase transition at T-0 around 150 K reveals an isotropic gap selectively opening on one Fermi surface with finite warping. This band selectivity is incompatible with conventional gap opening mechanisms and suggests a role of Kondo-type proximity coupling in stabilizing the exotic phase for potential unconventional superconductivity.
Complex electronic phases in strongly correlated electron systems are manifested by broken symmetries in the low-energy electronic states. Some mysterious phases, however, exhibit intriguing energy gap opening without an apparent signature of symmetry breaking (e.g., high-T-C cuprates and heavy fermion superconductors). Here, we report an unconventional gap opening in a hetero-structured, iron-based superconductor Sr2VO3FeAs across a phase transition at T-0 similar to 150 K. Using angle-resolved photoemission spectroscopy, we identify that a fully isotropic gap opens selectively on one of the Fermi surfaces with finite warping along the interlayer direction. This band selectivity is incompatible with conventional gap opening mechanisms associated with symmetry breaking. These findings, together with the unusual field-dependent magneto-resistance, suggest that the Kondo-type proximity coupling of itinerant Fe electrons to localized V spin plays a role in stabilizing the exotic phase, which may serve as a distinct precursor state for unconventional superconductivity.

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