Journal
INORGANIC CHEMISTRY
Volume 55, Issue 15, Pages 7250-7256Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.inorgchem.6b00897
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Funding
- National Science Foundation [DMR-1507210]
- Office of Science, Office of Basic Energy Science, U.S. Department of Energy [DE-AC02-05CH11231]
- Direct For Mathematical & Physical Scien
- Division Of Materials Research [1507210] Funding Source: National Science Foundation
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Energy-efficient solid-state-lighting (SSL) technologies are rapidly developing, but the lack of stable, high-performance rare-earth free phosphors may impede the growth of the SSL market. One possible alternative is organic phosphor materials, but these can suffer from lower quantum yields and thermal instability compared to rare-earth phosphors. However, if luminescent organic chromophores can be built into a rigid metal organic framework, their quantum yields and thermal stability can be greatly improved. This Forum Article discusses the design of a group of such chromophore-based luminescent metal-organic frameworks with exceptionally high performance and rational control of the important parameters that influence their emission properties, including electronic structures of chromophore, coligands, metal ions, and guest molecules.
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