Journal
ORGANIC PROCESS RESEARCH & DEVELOPMENT
Volume 26, Issue 7, Pages 1900-1913Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.oprd.1c00413
Keywords
photobiocatalysis; cofactor recycling; H2O2 generation in situ; cascades; photoactive cofactor
Categories
Funding
- National Key Research and Development Program of China [2021YFC2102000]
- National Natural Science Foundation of China [91956128]
- Natural Science Foundation of Zhejiang Province [LY19B020014]
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This review provides an overview of recent progress in photobiocatalysis, including the regeneration of cofactors, generation of H2O2 in situ, cascades involving a photobiocatalytic transformation, and the photoinduced enzymatic reactions inspired by the photoactive cofactor within the enzyme.
Photocatalysis has emerged as a powerful tool to generate reactive intermediates under mild reaction conditions. The combination of photocatalysis and biocatalysis, possessing advantages of the reactivity of photocatalysts and the selectivity of enzymes, has received increasing attention for its potential to realize the green synthesis of value-added chemicals. This review provides an overview of recent progress in photobiocatalysis, including the regeneration of cofactors, generation of H2O2 in situ, cascades involving a photobiocatalytic transformation, and the photoinduced enzymatic reactions inspired by the photoactive cofactor within the enzyme.
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