4.8 Article

Thermodynamics of free and bound magnons in graphene

Journal

NATURE PHYSICS
Volume 18, Issue 1, Pages 37-+

Publisher

NATURE PORTFOLIO
DOI: 10.1038/s41567-021-01421-x

Keywords

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Funding

  1. US Department of Energy, Basic Energy Sciences Office, Division of Materials Sciences and Engineering [DE-SC0001819, DE-SC0019300]
  2. Gordon and Betty Moore Foundations EPiQS Initiative [GBMF9468]
  3. ARO [W911NF-14-1-0247]
  4. STC Center for Integrated Quantum Materials, National Science Foundation (NSF) [DMR-1231319]
  5. Department of Defense through the National Defense Science and Engineering Graduate Fellowship (NDSEG) program
  6. Harvard Quantum Initiative in Science and Engineering
  7. Harvard Quantum Initiative Seed Fund
  8. NSF Graduate Research Fellowship [DGE 1745303]
  9. Elemental Strategy Initiative by the MEXT, Japan [JPMXP0112101001]
  10. JSPS KAKENHI [JP20H00354]
  11. CREST, JST [JPMJCR15F3]
  12. NSF [ECS-0335765]

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The passage discusses the ferromagnetic phase observed in the quantum Hall effect and the study of related magnon excitations. By measuring the electron compressibility under the influence of magnons, a reduction in the gap of the quantum Hall state is revealed. The analysis suggests injected magnons bind with electrons and holes to form skyrmions, allowing the extraction of free magnon density, magnon chemical potential, and average skyrmion spin.
Symmetry-broken electronic phases support neutral collective excitations. For example, monolayer graphene in the quantum Hall regime hosts a nearly ideal ferromagnetic phase at specific filling factors that spontaneously breaks the spin-rotation symmetry(1-3). This ferromagnet has been shown to support spin-wave excitations known as magnons that can be electrically generated and detected(4,5). Although long-distance magnon propagation has been demonstrated via transport measurements, important thermodynamic properties of such magnon populations-including the magnon chemical potential and density-have not been measured. Here we present local measurements of electron compressibility under the influence of magnons, which reveal a reduction in the gap associated with the nu =1 quantum Hall state by up to 20%. Combining these measurements with the estimates of temperature, our analysis reveals that the injected magnons bind to electrons and holes to form skyrmions, and it enables the extraction of free magnon density, magnon chemical potential and average skyrmion spin. Our methods provide a means of probing the thermodynamic properties of charge-neutral excitations that are applicable to other symmetry-broken electronic phases.

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