4.8 Article

Fabrication and nanophotonic waveguide integration of silicon carbide colour centres with preserved spin-optical coherence

Journal

NATURE MATERIALS
Volume 21, Issue 1, Pages 67-+

Publisher

NATURE PORTFOLIO
DOI: 10.1038/s41563-021-01148-3

Keywords

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Funding

  1. Ion Beam Centre at Helmholtz-Zentrum Dresden-Rossendorf
  2. Swedish Research Council [2020-05444]
  3. Swedish Energy Agency [43611-1]
  4. EU [862721]
  5. Knut and Alice Wallenberg Foundation [KAW 2018.0071]
  6. UC Davis Summer GSR Award
  7. National Science Foundation [CAREER-2047564]
  8. EU-FET Flagship on Quantum Technologies [820394, 820445]
  9. European Research Council (ERC) grant SMel
  10. Max Planck Society
  11. German Research Foundation [SPP 1601, FOR 2724]
  12. German Federal Ministry of Education and Research (BMBF) [16KIS0867]
  13. Swedish Research Council [2020-05444] Funding Source: Swedish Research Council

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Optically addressable spin defects in silicon carbide (SiC) are a promising platform for quantum information processing, enabling high-fidelity spin qubit operations. However, degradation of spin-optical coherence after integration in nanophotonic structures poses a challenge for scalability towards large-scale quantum networks.
Colour centres are a promising quantum information platform, but coherence degradation after integration in nanostructures has hindered scalability. Here, the authors show that waveguide-integrated V-Si centres in SiC maintain spin-optical coherences, enabling nuclear high-fidelity spin qubit operations. Optically addressable spin defects in silicon carbide (SiC) are an emerging platform for quantum information processing compatible with nanofabrication processes and device control used by the semiconductor industry. System scalability towards large-scale quantum networks demands integration into nanophotonic structures with efficient spin-photon interfaces. However, degradation of the spin-optical coherence after integration in nanophotonic structures has hindered the potential of most colour centre platforms. Here, we demonstrate the implantation of silicon vacancy centres (V-Si) in SiC without deterioration of their intrinsic spin-optical properties. In particular, we show nearly lifetime-limited photon emission and high spin-coherence times for single defects implanted in bulk as well as in nanophotonic waveguides created by reactive ion etching. Furthermore, we take advantage of the high spin-optical coherences of V-Si centres in waveguides to demonstrate controlled operations on nearby nuclear spin qubits, which is a crucial step towards fault-tolerant quantum information distribution based on cavity quantum electrodynamics.

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