4.8 Article

Charge-density-wave-driven electronic nematicity in a kagome superconductor

Journal

NATURE
Volume 604, Issue 7904, Pages 59-+

Publisher

NATURE PORTFOLIO
DOI: 10.1038/s41586-022-04493-8

Keywords

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Funding

  1. National Key R&D Program of the MOST of China [2017YFA0303000]
  2. National Natural Science Foundation of China [11888101, 12034004, 12074364]
  3. Strategic Priority Research Program of the Chinese Academy of Sciences [XDB25000000]
  4. Anhui Initiative in Quantum Information Technologies [AHY160000]
  5. Collaborative Innovation Program of Hefei Science Center, CAS [2019HSC-CIP007]

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This study presents evidence for the existence of electronic nematicity in CsV3Sb5, providing new insights into the pairing mechanism in unconventional superconductors.
Electronic nematicity, in which rotational symmetry is spontaneously broken by electronic degrees of freedom, has been demonstrated as a ubiquitous phenomenon in correlated quantum fluids including high-temperature superconductors and quantum Hall systems(1,2). Notably, the electronic nematicity in high-temperature superconductors exhibits an intriguing entanglement with superconductivity, generating complicated superconducting pairing and intertwined electronic orders. Recently, an unusual competition between superconductivity and a charge-density-wave (CDW) order has been found in the AV(3)Sb(5) (A = K, Rb, Cs) family with two-dimensional vanadium kagome nets(3-8). Whether these phenomena involve electronic nematicity is still unknown. Here we report evidence for the existence of electronic nematicity in CsV3Sb5, using a combination of elastoresistance measurements, nuclear magnetic resonance (NMR) and scanning tunnelling microscopy/spectroscopy (STM/S). The temperature-dependent elastoresistance coefficient (m(11) minus m(12)) and NMR spectra demonstrate that, besides a C-2 structural distortion of the 2a(0) x 2a(0) supercell owing to out-of-plane modulation, considerable nematic fluctuations emerge immediately below the CDW transition (approximately 94 kelvin) and finally a nematic transition occurs below about 35 kelvin. The STM experiment directly visualizes the C-2-structure-pinned long-range nematic order below the nematic transition temperature, suggesting a novel nematicity described by a three-state Potts model. Our findings indicate an intrinsic electronic nematicity in the normal state of CsV3Sb5, which sets a new paradigm for revealing the role of electronic nematicity on pairing mechanism in unconventional superconductors.

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