4.8 Article

Strong Zero-Phonon Transition from Point Defect-Stacking Fault Complexes in Silicon Carbide Nanowires

Journal

NANO LETTERS
Volume 21, Issue 21, Pages 9187-9194

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acs.nanolett.1c03013

Keywords

silicon carbide; point defect; stacking fault; nanowire; Debye-Waller factor

Funding

  1. Research Foundation of Korea (MSIT) [NRF-2019M3E4A1078664, NRF-2020M3H3A1098869, NRF-2021R1A2C2006904]
  2. ITRC (Information Technology National Research Center) support program [IITP 2021-2020-0-01606]
  3. KIST Institutional Program [2E29580-19-146]
  4. EU QuantERA Nanospin project [National Research, Development and Innovation Office of Hungary (NKFIH)] [127902]
  5. National Quantum Technology Project (NKFIH) [2017-1.2.1-NKP-2017-00001]
  6. Quantum Information National Laboratory - Ministry for Innovation and Technology of Hungary via NKFIH
  7. National Excellence Program (NKFIH) [KKP129866]
  8. European Commission (QuanTelCO project) [862721]
  9. National Research Foundation of Korea [2019M3E4A1078664, 2020M3H3A1098869] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)

Ask authors/readers for more resources

The study found that point-planar defect complexes in silicon carbide nanowires exhibit outstanding optical properties, potentially enabling highly efficient quantum interactions between multiple qubits.
Crystallographic defects such as vacancies and stacking faults engineer electronic band structure at the atomic level and create zero- and two-dimensional quantum structures in crystals. The combination of these point and planar defects can generate a new type of defect complex system. Here, we investigate silicon carbide nanowires that host point defects near stacking faults. These point-planar defect complexes in the nanowire exhibit outstanding optical properties of high-brightness single photons (>360 kcounts/s), a fast recombination time (<1 ns), and a high Debye-Waller factor (>50%). These distinct optical properties of coupled point-planar defects lead to an unusually strong zero-phonon transition, essential for achieving highly efficient quantum interactions between multiple qubits. Our findings can be extended to other defects in various materials and therefore offer a new perspective for engineering defect qubits.

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