4.6 Article

Continuous Oil-Water Separation Using Polydimethylsiloxane-Functionalized Melamine Sponge

Journal

INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH
Volume 55, Issue 12, Pages 3596-3602

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acs.iecr.6b00234

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Funding

  1. Div Of Industrial Innovation & Partnersh
  2. Directorate For Engineering [1238318] Funding Source: National Science Foundation

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The development of absorbent materials with high selectivity for oils and organic solvents is of great ecological importance for removing pollutants from contaminated water sources. We have developed a facile solution-immersion process for creating polydimethylsiloxane (PDMS)-functionalized sponges for oil water separation. Sponge materials with densities ranging from 8 to 26 mg/cm(3) were investigated as candidate skeletons. After functionalization, the lowest-density melamine sponge exhibits superior superhydrophobic and superoleophilic properties, absorption capacity, oil water selectivity, and absorption recyclability. Via suction through such a functionalized sponge, we have experimentally demonstrated that various kinds of oils can be continuously separated from immiscible liquid mixtures without any water uptake. The widely available raw materials (melamine sponge and PDMS solution) and simple synthesis steps yield a cost-effective and scalable process for fabrication of absorbent materials that can be readily adopted for the cleanup of oil spills and industrial chemical leakage of low-surface-tension solvents that are immiscible with water.

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