Journal
JOURNAL OF ORGANIC CHEMISTRY
Volume 87, Issue 5, Pages 3596-3604Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.joc.1c03151
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Funding
- Natural Science Foundation of Zhejiang Province of China [LQ21B060001]
- Leading Innovative and Entrepreneur Team Introduction Program of Zhejiang [2019R01005]
- China Postdoctoral Science Foundation [2021M692859]
- Taizhou University Research Project [2019PY029]
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We report the first example of a visible-light-induced approach for the synthesis of spiroquinazolin(thi)ones, which features an eco-friendly energy source and solvent, metal-free catalysts, step- and atom- economy, a relay catalysis strategy, air as a green oxidant, mild conditions, and easily accessible starting materials.
The multicomponent-multicatalyst reaction ((MC)R-2) and visible-light catalysis have emerged as green and powerful strategies for achieving ideal syntheses. Here, we report the first example of a visible-light-induced approach toward spiroquinazolin(thi)ones. This (MC)R-2 features an eco-friendly energy source and solvent, metal-free catalysts, step- and atom- economy, a relay catalysis strategy, air as green oxidant, mild conditions, and easily accessible starting materials.
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